Abstract:Superconducting properties change in confined geometries. Here we study the effects of strong confinement in nanosized Pb-islands on Si(111) 7×7. Small hexagonal islands with diameters less than 50 nm and a uniform height of 7 atomic layers are formed by depositing Pb at low temperature and annealing at 300 K. We measure the tunneling spectra of individual Pb-nanoislands using a low-temperature scanning tunneling microscope operated at 0.6 K, and follow the narrowing of the superconducting gap as a function of… Show more
“…[ 27,28 ] Then, 20‐nm‐thick Pb was deposited on single‐crystalline graphene by electron beam evaporation (Experimental Section; Figure S2, Supporting Information). Owing to the poor wettability of graphene [ 8,11 ] and the low melting point of Pb, [ 29,30 ] the deposited Pb is prone to being randomly distributed into irregular disconnected nanoislands, as suggested by cross‐sectional transmission electron microscopy (TEM, Figure a) and plan‐view scanning electron microscopy (SEM) in Figure 1b. TEM–energy dispersive X‐ray spectroscopy (TEM–EDS, Figure 1d) further proves that Pb nanoislands are completely disconnected from each other.…”
Disorder-induced Griffiths singularity of quantum phase transition (QPT) is a crucial issue in 2D superconductors (2DSC). In a superconducting system, the strength of disorder is found to be associated with the vortex pinning energy, which is closely related to the quantum Griffiths singularity; however, a direct study to elucidate the role of vortex pinning energy on the quantum Griffiths singularity in 2DSC remains to be undertaken. Here, an artificial 2DSC system is designed by randomly depositing superconducting nanoislands on 2Delectron gas (2DEG). Quantum Griffiths singularity is present in a graphene/Pb-islands-array hybrid, where the superconducting behavior transits to weakly localized metallic behavior induced by the vertical magnetic field and exhibits critical behavior with a diverging dynamical critical exponent approaching zero temperature. Compared to the study of graphene/Sn-islands-array hybrid where the sharp QPT is observed, the vortex pinning energy acquired from the Arrhenius plot analysis is greater in graphene/Pb-islands-array hybrid, which may contribute to the presence of the quantum Griffiths singularity. This work may provide a comprehensive interpretation of the QPT in 2DSC.
“…[ 27,28 ] Then, 20‐nm‐thick Pb was deposited on single‐crystalline graphene by electron beam evaporation (Experimental Section; Figure S2, Supporting Information). Owing to the poor wettability of graphene [ 8,11 ] and the low melting point of Pb, [ 29,30 ] the deposited Pb is prone to being randomly distributed into irregular disconnected nanoislands, as suggested by cross‐sectional transmission electron microscopy (TEM, Figure a) and plan‐view scanning electron microscopy (SEM) in Figure 1b. TEM–energy dispersive X‐ray spectroscopy (TEM–EDS, Figure 1d) further proves that Pb nanoislands are completely disconnected from each other.…”
Disorder-induced Griffiths singularity of quantum phase transition (QPT) is a crucial issue in 2D superconductors (2DSC). In a superconducting system, the strength of disorder is found to be associated with the vortex pinning energy, which is closely related to the quantum Griffiths singularity; however, a direct study to elucidate the role of vortex pinning energy on the quantum Griffiths singularity in 2DSC remains to be undertaken. Here, an artificial 2DSC system is designed by randomly depositing superconducting nanoislands on 2Delectron gas (2DEG). Quantum Griffiths singularity is present in a graphene/Pb-islands-array hybrid, where the superconducting behavior transits to weakly localized metallic behavior induced by the vertical magnetic field and exhibits critical behavior with a diverging dynamical critical exponent approaching zero temperature. Compared to the study of graphene/Sn-islands-array hybrid where the sharp QPT is observed, the vortex pinning energy acquired from the Arrhenius plot analysis is greater in graphene/Pb-islands-array hybrid, which may contribute to the presence of the quantum Griffiths singularity. This work may provide a comprehensive interpretation of the QPT in 2DSC.
“…Over the past three decades, great interests have been focused on the electronic transport properties of granular composites consisting of superconductors and insulators . The interests were firstly aroused by the enhancement of the superconducting transition temperature and critical magnetic field of nanostructured superconducting materials .…”
We studied the electronic transport properties of Pb x (SiO 2 ) 1Àx nanogranular films with Pb volume fraction x ranging from $0.51 to $0.87 and thickness t > 500 nm. It has been found that those x 0 0.60 films reveal metallic behavior at normal state and change to superconductors below $7 K, while those x 0.53 films show insulator properties over the whole measured temperature range. The quasireentrant superconductivity behaviors were observed in the films with intermediate x values, x ' 0.54 and 0.57. It is found that the critical metal volume fraction x s c for superconductorinsulator transition is almost identical to the percolation threshold for metal-insulator transition. For the film with x just above x s c , the superconducting states can preserve to relative high temperatures even at a magnetic field with magnitude of 9 T, and the upper critical field at zero temperature is estimated to be close to the Pauli limit ($15 T). Our results establish a key element for the high field applications of superconducting material.
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Research Letter1700070 (4 of 5) Y.-J. Xi et al.: Quasireentrant superconductivity and enhanced critical field in granular Pb-SiO 2
“…This behavior generally can be fitted by a function as derived from the Ginzburg–Landau theory [ 50 ] and yields with nm T. A similar value has been reported for Pb islands on Si(111) for a range of smaller diameters, although the authors modify the function to to account for an effective superconducting area slightly different to the topographic one. [ 61 ] In the present study, the diameter independent offset is fitted to nm with nm T. However, the deviation remains small compared to the observed spread of critical fields. We do not observe vortex formation in our measurements up to effective diameters of ≈70 nm (see Figure S3c–f, Supporting Information, for more details about Δ and B c as function of island size).…”
Nanodevices based on hybrid graphene-superconductor structures have recently attracted much attention owing to both fundamental and application aspects. However, atomic-level investigations of proximity-induced superconductivity in graphene, especially on technologically relevant substrates remain rare. Here, the atomic-scale study of electronic properties and the superconducting proximity effect in hydrogen-intercalated single-layer graphene on SiC decorated with epitaxial lead (Pb) islands is reported. The graphene layer is thoroughly characterized by means of Landau level spectroscopy which confirms its quasi-free-standing nature. Scanning tunneling spectroscopy performed at 1.8 K on the graphene layer in the vicinity of Pb islands shows a reduced superconducting gap of gr = 0.20(1) meV, which points to a graphene/superconductor junction of moderate transparency. The variations of the proximity-induced superconducting gap on graphene are measured as function of spatial position as well as of magnetic field strength. Spatially resolved measurements yield a coherence length of about 175 nm in the graphene monolayer. The study provides a foundation for realization of graphene-superconductor heterostructures on large-scale SiC(0001) wafers suitable for future technological applications.
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