This study proposes a novel four-way
plasma-catalytic removal of
particulate matter, nitrogen oxides, hydrocarbons, and carbon monoxide
without external heating using a pulsed dielectric barrier discharge
reactor combined with Au/CaSO4/γ-Al2O3 catalyst balls. With the optimized amount of Au and CaSO4, over 90% of particulate matter, 40% of nitrogen oxides,
and nearly 100% of hydrocarbons were removed from the diesel engine
exhaust, while the increase of carbon monoxide concentration due to
the oxidation of particulate matter and hydrocarbons and the decomposition
of carbon dioxide were minimized. Importantly, the performance of
the plasma-catalytic reactor was maintained without decline for the
duration of the experiment (7 h) with an attractive cost/performance
ratio. These findings offer a new approach to the simultaneous treatment
of diesel exhausts and provide a novel concept for the design of a
practical and compact after-treatment device for the diesel engine
exhaust gases.