2016
DOI: 10.1021/acs.nanolett.6b01558
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Broadband Enhancement of Spontaneous Emission in Two-Dimensional Semiconductors Using Photonic Hypercrystals

Abstract: The low quantum yield observed in two-dimensional semiconductors of transition metal dichalcogenides (TMDs) has motivated the quest for approaches that can enhance the light emission from these systems. Here, we demonstrate broadband enhancement of spontaneous emission and increase in Raman signature from archetype two-dimensional semiconductors: molybdenum disulfide (MoS2) and tungsten disulfide (WS2) by placing the monolayers in the near field of a photonic hypercrystal having hyperbolic dispersion. Hypercry… Show more

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Cited by 98 publications
(80 citation statements)
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References 28 publications
(41 reference statements)
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“…Several experiments have successfully demonstrated the spontaneous emission modification and related applications using HMMs . For example, Figure a depicts the dependent relation of the CdSe/ZnS quantum dot lifetime dispersed on the metal–dielectric multilayer structures to emitting wavelength.…”
Section: D Bulk Hyperbolic Metamaterialsmentioning
confidence: 99%
See 1 more Smart Citation
“…Several experiments have successfully demonstrated the spontaneous emission modification and related applications using HMMs . For example, Figure a depicts the dependent relation of the CdSe/ZnS quantum dot lifetime dispersed on the metal–dielectric multilayer structures to emitting wavelength.…”
Section: D Bulk Hyperbolic Metamaterialsmentioning
confidence: 99%
“…Compared with other optical metamaterials, like chiral and split ring resonator–based metamaterials, HMMs have advantages of relative ease of fabrication at optical frequencies, broadband nonresonant and 3D bulk responses, and flexible wavelength tunability. As a result, HMMs have attracted widespread interest and become a good multifunctional platform for many exotic applications, such as optical negative refraction and light beam steering, subdiffraction‐limited imaging and nanolithography, spontaneous and thermal emission engineering, ultrasensitive optical, biological, and chemical sensing, omnidirectional and broadband optical absorption …”
Section: Introductionmentioning
confidence: 99%
“…It is noteworthy that the hyperbolic medium can either be a natural material with hyperbolic dispersion, such as bismuth [32], or an artificial one, i.e., HMM [31]. The photonic hypercrystals have also perceptible potential applications, such as guiding [31] and the broadband enhancement of spontaneous emission [33]. Moreover, the multilayered structure of the graphene-hBN subwavelength stack can also be considered as a hypercrystal, as far as the effective medium theory (EMT) does not break down.…”
Section: Introductionmentioning
confidence: 99%
“…et al . manuscript submitted), spontaneous emission engineering1617182930 and ultrafast switching20. In addition, the large momentum of BPPs has found use in asymmetric transmission devices31 and in HMM-clad waveguides with highly tailorable modal dispersion32333435.…”
mentioning
confidence: 99%
“…For example, one-dimensional rectilinear gratings16 and so-called hyper-crystal29 gratings made by focused ion beam were used to show emission enhancement of organic dyes and 2D transition metal dichalcogenides, respectively. In addition, nanohole array gratings17 and bullseye18 gratings made by electron-beam lithography (EBL) and dry etching were used with dyes and quantum dots, respectively.…”
mentioning
confidence: 99%