Ultrareliable and low-latency connection (URLLC) is one of the novel features in 5G networks and subsequent generations, in which it targets to fulfill stringent requirements on data rates, reliability, and availability. Moreover, the multiconnectivity concept is introduced to meet these requirements, where multiple different technologies are connected simultaneously, and the data packet is duplicated and transmitted from multiple transmitters. To this end, in this paper, we present an analysis, model, and method to ensure the reliability of data delivery when organizing URLLC in 5G networks. In addition, a new approach based on the organization of multiple connections (multiconnectivity) and duplication of transmitted data is considered. Further, an analytical model is presented for assessing the probability of failure, taking into account the traffic intensity, the probability of failure of elements, and the number of used connections. Moreover, an efficient method is proposed for increasing the reliability of data delivery by optimizing the number of connections. Further, a multiconnectivity-based URLLC model has been built for evaluating the proposed method and verifies that the optimal number of routes for data delivery between the user and the point of service can be obtained, where the probability of losses and equipment reliability are jointly considered. Finally, detailed analysis of results shown that with “equal” routes in terms of load (with an equally probable traffic distribution) and the probability of equipment failure, the optimal number of routes can be found, at which the minimum probability of losses is achieved.