Application of the hydrological model chain of the RODOS decision support system for nuclear emergencies to the analysis of possible consequences of severe accident

Pylypenko, Oleksandr; Kivva, Sergii; Kopka, Piotr; Potempski, S.; Wojciechowicz, H.; Zheleznyak, Mark

doi:10.1016/j.anucene.2023.109823

Annals of Nuclear Energy

2023

DOI: 10.1016/j.anucene.2023.109823

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Application of the hydrological model chain of the RODOS decision support system for nuclear emergencies to the analysis of possible consequences of severe accident

Oleksandr Pylypenko

Sergii Kivva

Piotr Kopka

et al.

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A Cucurbit[8]uril‐Based Supramolecular Framework Material for Reversible Iodine Capture in the Vapor Phase and Solution

Lu,

Yu,

Zhang

et al. 2023

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The safe and efficient management of hazardous radioactive iodine is significant for nuclear waste reprocessing and environmental industries. A novel supramolecular framework compound based on cucurbit[8]uril (Q[8]) and 4‐aminopyridine (4‐AP) is reported in this paper. In the single crystal structure of Q[8]‐(4‐AP), two 4‐AP molecules interact with the outer surface of Q[8] and the two other 4‐AP molecules are encapsulated into the Q[8] cavity to form the self‐assembly Q[8]‐(4‐AP). Iodine adsorption experiments show that the as‐prepared Q[8]‐(4‐AP) not only has a high adsorption capacity (1.74 g· g−1) for iodine vapor but also can remove the iodine in the organic solvent and the aqueous solution with the removal efficiencies of 95% and 91%, respectively. The presence of a large number of hydrogen bonds between the iodine molecule and the absorbent, as seen in the single crystal structure of iodine‐loaded Q[8]‐(4‐AP) (I2@Q[8]‐(4‐AP)), is thought to be responsible for the exceptional iodine adsorption capacity of the material. In addition, the adsorption‐desorption tests reveal that the self‐assembly material has no significant loss of iodine capture capacity after five cycles, indicating that it has sufficient reusability.

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A Cucurbit[8]uril‐Based Supramolecular Framework Material for Reversible Iodine Capture in the Vapor Phase and Solution

Lu,

Yu,

Zhang

et al. 2023

Small

View full text Add to dashboard Cite

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Application of the hydrological model chain of the RODOS decision support system for nuclear emergencies to the analysis of possible consequences of severe accident

Cited by 1 publication

References 33 publications

A Cucurbit[8]uril‐Based Supramolecular Framework Material for Reversible Iodine Capture in the Vapor Phase and Solution

A Cucurbit[8]uril‐Based Supramolecular Framework Material for Reversible Iodine Capture in the Vapor Phase and Solution

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