Antisite Disorder Induced Exchange Bias Effect and Spin Glass State in La2− X Sm X Nimno6

Hissariya, Raman; Sathe, Vasant; Mishra, Shrawan

doi:10.2139/ssrn.4305930

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“…The small observed hysteresis could be due to frustration in the structure. In recent times, there has been significant interest in exploring and understanding the effects of exchange bias (EB) in structurally inhomogeneous systems with various combinations of magnetic cations [30][31][32][38][39][40][41]. In the exchange bias effect, the field-cooled (FC) M-H loops show a shift along the magnetic field axis, and this is used in several technological applications, such as magnetic recording read heads [42], random access memories [43], and other spintronics devices [44,45].…”

Section: Resultsmentioning

confidence: 99%

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Magnetism and Exchange Bias Properties in Ba2ScRuO6

2023

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This paper presents structural, detailed magnetic, and exchange bias studies in polycrystalline Ba2ScRuO6 synthesized at ambient pressure. In contrast to its strontium analogue, this material crystallizes in a 6L hexagonal structure with space group P3¯m1. The Rietveld refinement using the room-temperature powder XRD pattern suggests a Ru-Sc disorder in the structure. The temperature variation of the DC electrical resistivity highlights a semiconducting behavior with the electron conduction corresponding to Mott’s 3D variable range hopping (VRH) model. The detailed magnetization measurements show that Ba2ScRuO6 develops antiferromagnetic ordering at TN≈ 9 K. Interestingly, below 9 K (TN), the field-cooled magnetic field variation (FC) of the magnetization curves highlights an exchange bias effect in the sample. The exchange bias field reaches a maximum value of 1.24 kOe at 2 K. The exchange bias effect below the magnetic ordering temperature can be attributed to the inhomogeneous magnetic correlations due to the disorder in the structure. Remarkably, the appearance of a large exchange bias field in Ba2ScRuO6 indicates that inhomogeneous hexagonal double perovskites are a promising class to explore new materials having potential applications in spintronics.

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Section: Resultsmentioning

confidence: 99%

“…The antisite disorder in LaSrCoFeO 6 shows a large exchange bias effect with an exchange bias field of 1.2 kOe at 5 K [31]. The antisite disorder in Sm-doped La 2 NiMnO 6 triggers an exchange bias and a spin glass effect [32].…”

Section: Introductionmentioning

confidence: 96%