2012
DOI: 10.1063/1.4730444
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Angular emission of ions and mass deposition from femtosecond and nanosecond laser-produced plasmas

Abstract: We investigated the angular distribution of ions and atoms emanating from femto- and nanosecond laser-produced metal plasmas under similar laser fluence conditions. For producing plasmas, aluminum targets are ablated in vacuum employing pulses from a Ti:Sapphire ultrafast laser (40 fs, 800 nm) and an Nd:YAG laser (6 ns, 1064 nm). The angular distribution of ion emission as well as the kinetic energy distribution is characterized by a Faraday cup, while a quartz microbalance is used for evaluating deposited mas… Show more

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Cited by 64 publications
(56 citation statements)
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“…At the high end of the fluence range, the larger low-energy peak attains such heights and widths that the high-energy shoulder becomes indistinguishable from it. This high-energy feature is also visible in other ablation experiments with pulse durations in the fs-ps range 15,17 and has been ascribed to the occurrence of an ambipolar field, resulting from a space-charge layer formed by electrons above the surface. This field accelerates some of the ions towards higher energies.…”
Section: B Peak Fluence Dependencementioning
confidence: 63%
See 1 more Smart Citation
“…At the high end of the fluence range, the larger low-energy peak attains such heights and widths that the high-energy shoulder becomes indistinguishable from it. This high-energy feature is also visible in other ablation experiments with pulse durations in the fs-ps range 15,17 and has been ascribed to the occurrence of an ambipolar field, resulting from a space-charge layer formed by electrons above the surface. This field accelerates some of the ions towards higher energies.…”
Section: B Peak Fluence Dependencementioning
confidence: 63%
“…13 Since the 1990s, many experiments have been performed and models developed 2,3 for laser-matter interaction at this particular time scale. Target materials used are metals such as gold, silver, copper, and aluminum, 5,12,[14][15][16][17][18][19][20][21] and non-metals such as silicon [22][23][24][25] and metal oxides, [26][27][28] among others. 29,30 Most of these studies are conducted in a femtosecond pulse length range from 50 fs up to approximately 1 ps and a pulse fluence up to 10 J/cm 2 .…”
Section: Introductionmentioning
confidence: 99%
“…Moreover, it is very interesting to note that scotch tests demonstrate that the films show an excellent adherence even at such large thickness and deposition rates. The production of films with such a large thickness can be attributed to the narrow angular distribution of the ablated material plume, which is well-known to be induced by two different laser parameters: short pulse duration [27] and large laser spot size [28]. All the depositions were carried out with an ultra-short pulse duration (5 ps) but also with a relatively large spot size, which resulted in a very directional plume towards the substrate surface.…”
Section: Resultsmentioning
confidence: 99%
“…Unlike ns LPP, the larger N e values found at closer distances in fs LPP are due to efficient material ablation via improved energy coupling between laser and the target [10]. This allows more ablated particles to be confined along the axial direction [37,38]. Moreover, confinement along the expansion direction increases the number density at higher pressures.…”
Section: Effect Of Pulse Width On T E and N Ementioning
confidence: 99%