In this study, the effects of tree species, tissue types, and tree size on the carbon concentration were studied, and the two additive systems, one with tree diameter (D), and the other with both D and tree height (H), were developed to estimate the stem, root, branch, and foliage carbon content of 10 broadleaf species in northeast China. The coefficients of the two systems were estimated with the nonlinear seemingly unrelated regression (NSUR), while the heteroscedasticity of the model residual was solved with the weight function. Our results showed that carbon concentrations varied along with tree species and size; the tissues and foliage contained higher carbon concentration than other observed tissues. The two additive carbon equation systems exhibited good predictive and fitting performance, with Ra2 > 0.87, average prediction error of approximately 0, and small average absolute error and absolute error percentage. The carbon equation system constructed with D and H exhibited better fit and performance, particularly for the stem and total carbon. Thus, the additive carbon equation systems estimated the tree carbon of 10 broadleaf species more accurately. These carbon equations can be used to monitor the carbon pool sizes for natural forests in the Chinese National Forest Inventory.