Ionic
polymer–metal composites (IPMC), one of the most popular
materials in the field of artificial muscle research, have attracted
much attention because of their high flexibility, low drive voltage
(<10 V), high force density, large deformation, and so forth. However,
the results show that the serious electrode fatigue crack and water
loss of traditional IPMC greatly decrease its fatigue life and limit
the practical application. In this study, we developed a novel liquid
metal composite electrode. A layer of eutectic gallium–indium
alloy (EGaIn) liquid metal was applied to the surface of the platinum
electrode of the IPMC using a mask. Because of the good self-healing
performance of the liquid metal, it is expected to solve the above
problems of resistance increase and water loss caused by cracks. It
turns out that the prepared EGaIn/Pt-IPMC exhibits a driving force
up to 120 mN and maximum fatigue life of about 25,000 s at a driving
voltage of 3 V. Compared with the best work reported, the fatigue
strength of EGaIn/Pt-IPMC was increased by about 210%, and the maximum
driving force of EGaIn/Pt-IPMC prepared by a single-layer basement
membrane was between the IPMC prepared by 4–6 layer basement
membrane. The electromechanical properties were significantly improved,
and it is expected to realize a series of bionic applications.