We investigate antireflection (AR) coating materials for two different operation lasing regimes requiring broad spectral bandwidth. We characterize high-power continuous-wave (CW) wavelength-tunable vertical-externalcavity surface-emitting semiconductor lasers and their passive mode-locking capabilities when using semiconductor saturable absorber mirrors. One laser gain design was investigated with different single dielectric layers as AR coatings. The dielectric coating materials used were SiO 2 , Al 2 O 3 , Ta 2 O 5 , and TiO 2. The AR coating was designed to reduce pump reflection and increase the confinement factor of the microcavity. Average power of 4.6 W in CW and a total wavelength tuning range of 42 nm has been observed with the SiO 2-coated structure. The shortest pulse of 708 fs was also observed for the SiO 2-coated structure, with a corresponding CW wavelength tuning range of 36 nm.