2012
DOI: 10.5194/acpd-12-13515-2012
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A three-dimensional variational data assimilation system for multiple aerosol species with WRF/Chem and an application to PM<sub>2.5</sub> prediction

Abstract: A three-dimensional variational data assimilation (3-DVAR) algorithm for aerosols in a WRF/Chem model is presented. The WRF/Chem model uses the MOSAIC (Model for Simulating Aerosol Interactions and Chemistry) scheme, which explicitly treats eight major species (elemental/black carbon, organic carbon, nitrate, sulfate, chloride, ammonium, sodium, and the sum of other inorganic, inert mineral and metal species) and represents size distributions using a sectional method with four size bins. The 3-DVAR sche… Show more

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Cited by 21 publications
(42 citation statements)
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“…Data assimilation of ground‐based observational networks has been tested for aerosol prediction. For example, several studies have tested the assimilation of ground‐based particulate matter (PM) observations with most using optimal interpolation or variational methods [ Kahnert , ; Tombette et al , ; Pagowski et al , ; Schwartz et al , ; Jiang et al , ; Li et al , ; Lee et al , ]. Pagowski and Grell [] and Schwartz et al [] used ground‐based PM 2.5 measurements from the Environmental Protection Agency's AIRnow network for regional fine aerosol predictions in the United States using several different DA methods.…”
Section: Introductionmentioning
confidence: 99%
“…Data assimilation of ground‐based observational networks has been tested for aerosol prediction. For example, several studies have tested the assimilation of ground‐based particulate matter (PM) observations with most using optimal interpolation or variational methods [ Kahnert , ; Tombette et al , ; Pagowski et al , ; Schwartz et al , ; Jiang et al , ; Li et al , ; Lee et al , ]. Pagowski and Grell [] and Schwartz et al [] used ground‐based PM 2.5 measurements from the Environmental Protection Agency's AIRnow network for regional fine aerosol predictions in the United States using several different DA methods.…”
Section: Introductionmentioning
confidence: 99%
“…Common DA methods are the optimal interpolation (OI)/3-dimensional variational (3D-Var) method (Daley, 1991), the ensemble Kalman filter (EnKF) (Evensen, 2009) and the 4-dimensional variational (4D-Var) method (Le Dimet and Talagrand, 1986). Following efforts in DA for trace gas modelling (Austin, 1992;Fisher and Lary, 1995;Elbern and Schmidt, 1999), in recent years, DA has been increasingly applied to aerosol forecasts (Collins et al, 2001;Benedetti et al, 2009;Tombette et al, 2009;Pagowski et al, 2010;Li et al, 2013;.…”
Section: Introductionmentioning
confidence: 99%
“…They showed a potentially powerful impact of the future lidar networks for PM 10 forecasts. Li et al (2013) used the OI for multiple aerosol species and for prediction of PM 2.5 in the Los Angeles basin. The OI method was also employed in a mesoscale numerical weather prediction system (GRAPES/CUACE_Dust) to study dust aerosol assimilation in eastern Asian (Wang and Niu, 2013).…”
Section: Introductionmentioning
confidence: 99%
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“…The 4D‐LETKF was also implemented to assimilate MODIS Dark Target and Deep Blue AOTs to improve dust analyses and forecasts with assimilations at four time slots (every 6 hr) for a 24‐hr assimilation window (Di Tomaso et al, ). In addition to the assimilation of routine satellite‐based and ground‐based AOTs, sparse surface or aircraft observations of aerosol mass concentrations, such as PM 2.5 and PM 10 , were also successfully assimilated to correct model simulations with variational or ensemble‐based methods (Li et al, ; Pagowski et al, ; Pagowski & Grell, ; Peng et al, ; Zang et al, ).…”
Section: Introductionmentioning
confidence: 99%