Abstract. A new cloud microphysical scheme including a detailed parameterization for
aerosol-driven ice formation in cirrus clouds is implemented in the global
ECHAM/MESSy Atmospheric Chemistry (EMAC) chemistry–climate model and
coupled to the third generation of the Modal Aerosol Dynamics model for Europe adapted for global applications (MADE3) aerosol submodel. The new
scheme is able to consistently simulate three regimes of stratiform clouds –
liquid, mixed-, and ice-phase (cirrus) clouds – considering the activation of
aerosol particles to form cloud droplets and the nucleation of ice
crystals. In the cirrus regime, it allows for the competition between
homogeneous and heterogeneous freezing for the available supersaturated water
vapor, taking into account different types of ice-nucleating particles, whose
specific ice-nucleating properties can be flexibly varied in the model
setup. The new model configuration is tuned to find the optimal set of
parameters that minimizes the model deviations with respect to
observations. A detailed evaluation is also performed comparing the model
results for standard cloud and radiation variables with a comprehensive set of
observations from satellite retrievals and in situ measurements. The
performance of EMAC-MADE3 in this new coupled configuration is in line with
similar global coupled models and with other global aerosol models featuring
ice cloud parameterizations. Some remaining discrepancies, namely a high
positive bias in liquid water path in the Northern Hemisphere and
overestimated (underestimated) cloud droplet number concentrations over the
tropical oceans (in the extratropical regions), which are both
a common problem in these kinds of models, need to be taken into account in
future applications of the model. To further demonstrate the readiness of the
new model system for application studies, an estimate of the anthropogenic
aerosol effective radiative forcing (ERF) is provided, showing that EMAC-MADE3
simulates a relatively strong aerosol-induced cooling but within the range
reported in the Intergovernmental Panel on Climate Change (IPCC) assessments.