Amorphous InGaZnO
x
(a-IGZO) thin-film transistors (TFTs) are currently
used in flat-panel displays due to their beneficial properties. However,
the mobility of ∼10 cm2/(V s) for the a-IGZO TFTs
used in commercial organic light-emitting diode TVs is not satisfactory
for high-resolution display applications such as virtual and augmented
reality applications. In general, the electrical properties of amorphous
oxide semiconductors are strongly dependent on their chemical composition;
the indium (In)-rich IGZO achieves a high mobility of 50 cm2/(V s). However, the In-rich IGZO TFTs possess another issue of negative
threshold voltage owing to intrinsically high carrier density. Therefore,
the development of an effective way of carrier density suppression
in In-rich IGZO will be a key strategy to the realization of practical
high-mobility a-IGZO TFTs. In this study, we report that In-rich IGZO
TFTs with vertically stacked InO
x
, ZnO
x
, and GaO
x
atomic
layers exhibit excellent performances such as saturation mobilities
of ∼74 cm2/(V s), threshold voltage of −1.3
V, on/off ratio of 8.9 × 108, subthreshold swing of
0.26 V/decade, and hysteresis of 0.2 V, while keeping a reasonable
carrier density of ∼1017 cm–3.
We found that the vertical dimension control of IGZO active layers
is critical to TFT performance parameters such as mobility and threshold
voltage. This study illustrates the potential advantages of atomic
layer deposition processes for fabricating ultrahigh-mobility oxide
TFTs.