The ''island of inversion'' nucleus 32 Mg has been studied by a (t, p) two neutron transfer reaction in inverse kinematics at REX-ISOLDE. The shape coexistent excited 0 þ state in 32 Mg has been identified by the characteristic angular distribution of the protons of the ÁL ¼ 0 transfer. The excitation energy of 1058 keV is much lower than predicted by any theoretical model. The low-ray intensity observed for the decay of this 0 þ state indicates a lifetime of more than 10 ns. Deduced spectroscopic amplitudes are compared with occupation numbers from shell-model calculations. The evolution of shell structure in exotic nuclei as a function of the proton (Z) and neutron (N) number is currently at the center of many theoretical and experimental investigations [1,2]. It has been realized that the interaction of the last valence protons and neutrons, in particular, the monopole component of the residual interaction between those nucleons, can lead to significant shifts in the single-particle energies, leading to the disappearance of classic shell closures and the appearance of new shell gaps [3]. A prominent example is the collapse of the N ¼ 20 shell gap in the neutron-rich oxygen isotopes where instead a new magic shell gap appears for 24 O at N ¼ 16 [4,5]. Recent work showed that the disappearance of the N ¼ 20 shell can be attributed to the monopole effect of the tensor force [3,6,7]. The reduced strength of the attractive interaction between the proton d 5=2 and the neutron d 3=2 orbitals causes the d 3=2 orbital to rise in energy and come closer to the f 7=2 orbital. In regions without pronounced shell closures correlations between the valence nucleons may become as large as the spacing of the single-particle energies. This can thus lead to particle-hole excitations to higher-lying single-particle states enabling deformed configurations to be lowered in energy. This may result in low-lying collective excitations, the coexistence of different shapes at low energies or even the deformation of the ground state for nuclei with the conventional magic number N ¼ 20. Such an effect occurs in the ''island of inversion'', one of most studied regions of exotic nuclei in the nuclear chart. In this region of neutron-rich nuclei around the magic number N ¼ 20 strongly deformed ground states in Ne, Na, and Mg isotopes have been observed [8-11]. Because of the reduction of the N ¼ 20 shell gap, quadrupole correlations can enable low-lying deformed 2p-2h intruder states from the fp shell to compete with spherical normal neutron 0p-0h states of the sd shell. In this situation the promotion of a neutron pair across the N ¼ 20 gap can result in deformed intruder ground states. Consequentially, the competition of two configurations can lead to the coexistence of spherical and deformed 0 þ states in the neutron-rich 30;32 Mg nuclei [12]. Coulomb excitation experiments have shown that 30 Mg has a rather small BðE2Þ value for the 0 þ gs ! 2 þ 1 transition [13,14] placing this nucleus outside the island of inversion. The excited deform...
In an experiment at the SISSI/LISE3 facility of GANIL, we have studied the decay of the two proton-rich nuclei 45 Fe and 48 Ni. We identified 30 implantations of 45 Fe and observed for the second time four implantation events of 48 Ni. In 17 cases, 45 Fe decays by two-proton emission with a decay energy of 1.154(16) MeV and a half-life of T 1/2 = 1.6 +0.5 −0.3 ms. The observation of 48 Ni and of its decay allows us to deduce a half-life of T 1/2 = 2.1 +2.1 −0.7 ms. One out of four decay events is completely compatible with two-proton radioactivity and may therefore indicate that 48 Ni has a two-proton radioactivity branch. We discuss all information now available on two-proton radioactivity for 45 Fe and 48 Ni and compare it to theoretical models.
The neutron-rich isotopes of cadmium up to the N ¼ 82 shell closure have been investigated by highresolution laser spectroscopy. Deep-uv excitation at 214.5 nm and radioactive-beam bunching provided the required experimental sensitivity. Long-lived isomers are observed in 127 Cd and 129 Cd for the first time. One essential feature of the spherical shell model is unambiguously confirmed by a linear increase of the 11=2 À quadrupole moments. Remarkably, this mechanism is found to act well beyond the h 11=2 shell. DOI: 10.1103/PhysRevLett.110.192501 PACS numbers: 21.10.Ky, 21.60.Cs, 31.15.aj, 32.10.Fn When first proposed, the nuclear shell model was largely justified on the basis of magnetic-dipole properties of nuclei [1]. The electric quadrupole moment could have provided an even more stringent test of the model, as it has a very characteristic linear behavior with respect to the number of valence nucleons [2,3]. However, the scarcity of experimental quadrupole moments at the time did not permit such studies. Nowadays, regardless of experimental challenges, the main difficulty is to predict which nuclei are likely to display this linear signature. The isotopes of cadmium, investigated here, proved to be the most revealing case so far. Furthermore, being in the neighborhood of the ''magic'' tin, cadmium is of general interest for at least two additional reasons. First, theory relies on nuclei near closed shells for predicting other, more complex systems. Second, our understanding of stellar nucleosynthesis strongly depends on the current knowledge of nuclear properties in the vicinity of the doubly magic tin isotopes [4]. Moreover, specific questions concerning the nuclear structure of the cadmium isotopes require critical evaluation, such as shell quenching [5,6], sphericity [7], deformation [8,9], or whether vibrational nuclei exist at all [10]. Some of these points will be addressed here quite transparently, while others require dedicated theoretical work to corroborate our conclusions. In this Letter we report advanced measurements by collinear laser spectroscopy on the very neutron-rich cadmium isotopes. Electromagnetic moments in these complex nuclei are found to behave in an extremely predictable manner. Yet, their description goes beyond conventional interpretation of the nuclear shell model.The measurements were carried out with the collinear laser spectroscopy setup at ISOLDE-CERN. High-energy protons impinging on a tungsten rod produced low-to medium-energy neutrons inducing fission in a uranium carbide target. Proton-rich spallation products, such as cesium, were largely suppressed in this manner. Further reduction of surface-ionized isobaric contamination was achieved by the use of a quartz transfer line [11], which allowed the more volatile cadmium to diffuse out of the target while impurities were retained sufficiently long to decay. Cadmium atoms were laser ionized, accelerated to an energy of 30 keV, and mass separated. The ion beam was injected into a gas-filled radio-frequency Paul trap [12]...
We report on the g-factor measurement of the first isomeric state in (16)43S27 [Ex=320.5(5) keV, T1/2=415(5) ns, and g=0.317(4)]. The 7/2- spin-parity of the isomer and the intruder nature of the ground state of the nucleus are experimentally established for the first time, providing direct and unambiguous evidence of the collapse of the N=28 shell closure in neutron-rich nuclei. The shell model, beyond the mean-field and semiempirical calculations, provides a very consistent description of this nucleus showing that a well deformed prolate and quasispherical states coexist at low energy.
At the radioactive ion beam facility REX-ISOLDE, neutron-rich zinc isotopes were investigated using lowenergy Coulomb excitation. These experiments have resulted in B(E2, 2 74,76 Zn and the determination of the energy of the first excited 2 + 1 states in 78,80 Zn. The zinc isotopes were produced by high-energy proton-(A = 74, 76, 80) and neutron-(A = 78) induced fission of 238 U, combined with selective laser ionization and mass separation. The isobaric beam was postaccelerated by the REX linear accelerator and Coulomb excitation was induced on a thin secondary target, which was surrounded by the MINIBALL germanium detector array. In this work, it is shown how the selective laser ionization can be used to deal with the considerable isobaric beam contamination and how a reliable normalization of the experiment can be achieved. The results for zinc isotopes and the N = 50 isotones are compared to collective model predictions and state-of-the-art large-scale shell-model calculations, including a recent empirical residual interaction constructed to describe the present experimental data up to 2004 in this region of the nuclear chart.
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