Boosting large-scale superconductor applications require nanostructured conductors with artificial pinning centres immobilizing quantized vortices at high temperature and magnetic fields. Here we demonstrate a highly effective mechanism of artificial pinning centres in solution-derived high-temperature superconductor nanocomposites through generation of nanostrained regions where Cooper pair formation is suppressed. The nanostrained regions identified from transmission electron microscopy devise a very high concentration of partial dislocations associated with intergrowths generated between the randomly oriented nanodots and the epitaxial YBa(2)Cu(3)O(7) matrix. Consequently, an outstanding vortex-pinning enhancement correlated to the nanostrain is demonstrated for four types of randomly oriented nanodot, and a unique evolution towards an isotropic vortex-pinning behaviour, even in the effective anisotropy, is achieved as the nanostrain turns isotropic. We suggest a new vortex-pinning mechanism based on the bond-contraction pairing model, where pair formation is quenched under tensile strain, forming new and effective core-pinning regions.
We demonstrate circular dichroism (CD) in the second harmonic generation (SHG) signal from chiral assemblies of G-shaped nanostructures made of gold. The arrangement of the G shapes is crucial since upon reordering them the SHG-CD effect disappears. Microscopy reveals SHG "hotspots" assemblies, which originate in enantiomerically sensitive plasmon modes, having the novel property of exhibiting a chiral geometry themselves in relation with the handedness of the material. These results open new frontiers in studying chirality.
Circularly polarized light is incident on a nanostructured chiral meta‐surface. In the nanostructured unit cells whose chirality matches that of light, superchiral light is forming and strong optical second harmonic generation can be observed.
We present a new electromagnetic phenomenon-the asymmetric second-harmonic generation from planar chiral structures. The effect consists in distinguishing the handedness of a chiral material by rotating the sample in an experiment involving solely linearly polarized light. This phenomenon originates in the surface plasmon resonance of chiral gold nanostructures, where homodyne interference of anisotropic and chiral electric and/or magnetic multipoles appears to play an important role.
It has been shown that a nanoliter chamber separated by a wall of asymmetric obstacles can lead to an inhomogeneous distribution of self-propelled microorganisms. Although it is well established that this rectification effect arises from the interaction between the swimmers and the noncentrosymmetric pillars, here we demonstrate numerically that its efficiency is strongly dependent on the detailed dynamics of the individual microorganism. In particular, for the case of run-and-tumble dynamics, the distribution of run lengths, the rotational diffusion, and the partial preservation of run orientation memory through a tumble are important factors when computing the rectification efficiency. In addition, we optimize the geometrical dimensions of the asymmetric pillars in order to maximize the swimmer concentration and we illustrate how it can be used for sorting by swimming strategy in a long array of parallel obstacles.
Vortex ratchet effect is investigated experimentally in the frequency range between 0.5 MHz and 2 GHz. The ratchet potential is provided by an array of about a quarter of a million nanoengineered asymmetric antidots in a Pb film. A square vortex lattice is stabilized at the first matching field, when each asymmetric antidot is occupied by a single vortex. We have found that ͑1͒ the transition from adiabatic to nonadiabatic cases occurring at about 1 MHz, above which the ratchet windows shift upwards with the applied frequency due to the fact that the time for a vortex to escape from the pinning potential is comparable to the period of the applied rf driving current I rf ; ͑2͒ a sudden V dc reversal at large I rf , which can be attributed to inertia effect; ͑3͒ the collective step-motor behavior in the MHz region, i.e., the vortex lattice moves forward by an integer number of the period of pinning array at each cycle of I rf ; and ͑4͒ very weak ratchet effect at several GHz, indicating the possibility of stronger inertia effects in the vortex motion at such high frequencies. These results reveal rich physics information in the nonadiabatic ratchet system and are of particular importance for particle separation and molecular motor in biology.
In high definition mapping of the plasmonic patterns on the surfaces of nanostructures, the diffraction limit of light remains an important obstacle. Here we demonstrate that this diffraction limit can be completely circumvented. We show that upon illuminating nanostructures made of nickel and palladium, the resulting surface-plasmon pattern is imprinted on the structures themselves; the hotspots (regions of local field enhancement) are decorated with overgrowths, allowing for their subsequent imaging with scanning-probe techniques. The resulting resolution of plasmon pattern imaging is correspondingly improved.
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