We generate attosecond pulse train (APT) in argon driven by the high repetition rate (HR) laser of the extreme light infrastructure-attosecond light pulse source (ELI-ALPS), providing 100 kHz, 80 W, 1030 nm, 40 fs pulses from a fiber chirped-pulse amplification (fiber-CPA) laser system. Under the current operating conditions of the high harmonic generation beamline (HR-GHHG), we observed the average pulse duration to be 395 as measured using the technique of reconstruction of attosecond beating by interference of two-photon transitions. The beamline uses an annular-shape laser beam so that the main part of the driving laser co-propagating with the APT can be eliminated by reflection on a holey mirror. An additional 100 nm aluminum foil is used to filter out the remaining laser and the low order harmonics, allowing 2 pJ APT with a bandwidth from 25 eV to 50 eV to be transported to the target position where the APT interacts with matter. The implementation of the HR-GHHG beamline in ELI-ALPS delivering attosecond pulse trains at 100 kHz paves the way for time-resolved experiments in the infrastructure, especially those that involve rare events and coincidence analysis, both of which need high statistics.
High-repetition rate attosecond pulse sources are indispensable tools for time-resolved studies of electron dynamics, such as coincidence spectroscopy and experiments with high demands on statistics or signal-to-noise ratio, especially in the case of solid and big molecule samples in chemistry and biology. Although with the high-repetition rate lasers, such attosecond pulses in a pump-probe configuration are possible to achieve, until now, only a few such light sources have been demonstrated. Here, by shaping the driving laser to an annular beam, a 100 kHz attosecond pulse train (APT) is reported with the highest energy so far (51 pJ/shot) on target (269 pJ at generation) among the high-repetition rate systems (>10 kHz) in which the attosecond pulses were temporally characterized. The on-target pulse energy is maximized by reducing the losses from the reflections and filtering of the high harmonics, and an unprecedented 19% transmission rate from the generation point to the target position is achieved. At the same time, the probe beam is also annular and low loss of this beam is reached by using another holey mirror to combine with the APT. The advantages of using an annular beam to generate attosecond pulses with a high-average power laser are demonstrated experimentally and theoretically. The effect of nonlinear propagation in the generation medium on the annular-beam generation concept is also analyzed in detail.
We present single-shot electron velocity-map images of nanoplasmas generated from doped helium nanodroplets and neon clusters by intense near-infrared and mid-infrared laser pulses. We report a large variety of signal types, most crucially depending on the cluster size. The common feature is a two-component distribution for each single-cluster event: a bright inner part with nearly circular shape corresponding to electron energies up to a few eV, surrounded by an extended background of more energetic electrons. The total counts and energy of the electrons in the inner part are strongly correlated and follow a simple power-law dependence. Deviations from the circular shape of the inner electrons observed for neon clusters and large helium nanodroplets indicate non-spherical shapes of the neutral clusters. The dependence of the measured electron energies on the extraction voltage of the spectrometer indicates that the evolution of the nanoplasma is significantly affected by the presence of an external electric field. This conjecture is confirmed by molecular dynamics simulations, which reproduce the salient features of the experimental electron spectra.
We generate high-order harmonics in a gaseous medium with tunable photon energy using time-domain interferometry of double pulses in a noncollinear generation geometry. The method is based on the fact that the generated harmonics inherit certain spectral properties of the driving laser. The two temporally delayed laser pulses, identical in all parameters, are produced by a custom-made split-and-delay unit utilizing wave-front splitting without a significant energy loss. The arrangement is easy to implement in any attosecond pulse generation beamline, and is suitable for the production of an extreme ultraviolet source with simply and quickly variable central photon energy, useful for a broad range of applications.
The dynamics and the decay processes of inner-shell excited atoms are of great interest in physics, chemistry, biology, and technology. The highly excited state decays very quickly through different channels, both radiative and non-radiative. It is therefore a long-standing goal to study such dynamics directly in the time domain. Using few-cycle infrared laser pulses, we investigated the excitation and ionization of inner-shell electrons through laser-induced electron re-collision with the original parent ions and measured the dependence of the emitted x-ray spectra on the intensity and ellipticity of the driving laser. These directly re-colliding electrons can be used as the initiating pump step in pump/probe experiments for studying core-hole dynamics at their natural temporal scale. In our experiment we found that the dependence of the x-ray emission spectrum on the laser intensity and polarization state varies distinctly for the two kinds of atomic systems. Relying on our data and numerical simulations, we explain this behavior by the presence of different excitation mechanisms that are contributing in different ratios to the respective overall x-ray emission yields. Direct re-collision excitation competes with indirect collisions with neighboring atoms by electrons having "drifted away" from the original parent ion.
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