Conventional spectroscopy uses classical light to detect matter properties through the variation of its response with frequencies or time delays. Quantum light opens up new avenues for spectroscopy by utilizing parameters of the quantum state of light as novel control knobs and through the variation of photon statistics by coupling to matter. This Roadmap article focuses on using quantum light as a powerful sensing and spectroscopic tool to reveal novel information about complex molecules that is not accessible by classical light. It aims at bridging the quantum optics and spectroscopy communities which normally have opposite goals: manipulating complex light states with simple matter e.g. qubits vs. studying complex molecules with simple classical light, respectively. Articles cover advances in the generation and manipulation of state-of-the-art quantum light sources along with applications to sensing, spectroscopy, imaging and interferometry.

Metasurfaces consisting of engineered dielectric or metallic structures provide unique solutions to realize exotic phenomena including negative refraction, achromatic focusing, electromagnetic cloaking, and so on. The intersection of metasurface and quantum optics may lead to new opportunities but is much less explored. Here, we propose and experimentally demonstrate that a polarization-entangled photon source can be used to switch ON or OFF the optical edge detection mode in an imaging system based on a high-efficiency dielectric metasurface. This experiment enriches both fields of metasurface and quantum optics, representing a promising direction toward quantum edge detection and image processing with remarkable signal-to-noise ratio.

Entanglement in multiple degrees of freedom has many benefits over entanglement in a single one. The former enables quantum communication with higher channel capacity and more efficient quantum information processing and is compatible with diverse quantum networks. Establishing multi-degree-of-freedom entangled memories is not only vital for high-capacity quantum communication and computing, but also promising for enhanced violations of nonlocality in quantum systems. However, there have been yet no reports of the experimental realization of multi-degree-of-freedom entangled memories. Here we experimentally established hyper- and hybrid entanglement in multiple degrees of freedom, including path (K-vector) and orbital angular momentum, between two separated atomic ensembles by using quantum storage. The results are promising for achieving quantum communication and computing with many degrees of freedom.

Multiphoton quantum states play a critical role in emerging quantum technologies and greatly improve our fundamental understanding of the quantum world. Integrated photonics is well recognized as an attractive technology offering great promise for the generation of photonic quantum states with high-brightness, tunability, stability, and scalability. Herein, we demonstrate the generation of multiphoton quantum states using a single-silicon nanophotonic waveguide. The detected four-photon rate reaches 0.34 Hz even with a low-pump power of 600 μW. This multiphoton quantum state is also qualified with multiphoton quantum interference, as well as quantum state tomography. For the generated four-photon states, the quantum interference visibilities are greater than 95%, and the fidelity is 0.78 ± 0.02. Furthermore, such a multiphoton quantum source is fully compatible with the on-chip processes of quantum manipulation, as well as quantum detection, which is helpful for the realization of large-scale quantum photonic integrated circuits (QPICs) and shows great potential for research in the area of multiphoton quantum science.

The silicon-on-chip (SOI) photonic circuit is a very promising platform for scalable quantum information technology for its low loss, small footprint, and its compatibility with CMOS as well as telecom communications techniques. Multiple multiplexed entanglement sources, including energytime, time-bin, and polarization-entangled sources based on 1-cm-length single-silicon nanowire, are all compatible with the (100-GHz) dense-wave-division-multiplexing (DWDM) system. Different methods, such as two-photon interference as well as Bell-inequality and quantum-state tomography, are used to characterize the quality of these entangled sources. Multiple entanglements are generated over more than five channel pairs with high raw (net) visibilities of around 97% (100%). The emission spectral brightness of these entangled sources reaches 4.210 5 /(s.nm.mW). The quality of the photon pair generated in continuous and pulse pump regimes are compared. The high quality of these multiplexed-entanglement sources makes them very promising for use in minimized quantum communications and computation systems.

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Integrated photonics is becoming an ideal platform for generating two-photon entangled states with high brightness, high stability and scalability. This high brightness and high quality of photon pair sources encourages researchers further to study and manipulate multi-photon entangled states. Here, we experimentally demonstrate frequency-degenerate four-photon entangled state generation based on a single silicon nanowire 1 cm in length. The polarization encoded entangled states are generated with the help of a Sagnac loop using additional optical elements. The states are analyzed using quantum interference and state tomography techniques. As an example, we show that the generated quantum states can be used to achieve phase super-resolution. Our work provides a method for preparing indistinguishable multi-photon entangled states and realizing quantum algorithms in a compact on-chip setting.

Spiral phase contrast is an important and convenient imaging processing technology in edge detection, and a broader field-of-view (FOV) of imaging is a long-pursuing aim to see more regions of the illumination objects. Compared with near-infrared (NIR) spectrum, the up-conversion imaging in visible spectrum benefits from the advantages of higher efficiency detection and lower potential speckle. FOV enhanced and spiral phase contrast up-conversion imaging processing methods by using second order nonlinear frequency up-conversion from NIR spectrum to visible spectrum in two different configurations are presented in this work. By changing the temperature of crystal, controllable spatial patterns of imaging with more than 4.5 times enhancement of FOV is realized in both configurations. Additionally, we present numerical simulations of the phenomenon, which agree well with the experimental observations. Our results provide a very promising way in imaging processing, which may be widely used in biomedicine, remote sensing and up-conversion monitoring.