M agnetic skyrmions are particle-like spin textures that have been observed in chiral bulk magnets 1-4 and asymmetric magnetic multilayers 5-14. Electrical currents and current-induced spin-orbit torques (SOTs) can be used to manipulate skyrmions in various metallic systems 2,7,8,10,14 , and such capabilities could be useful in the development of energy-efficient spintronic devices. Thermal effects can also be used to generate and manipulate skyrmions 15,16 , which could lead to the development of unconventional computing 17 and energy-harvesting 18 applications. These thermal effects are, however, difficult to observe in bulk samples and large-area films; therefore, microstructured devices need to be employed. Furthermore, the generation of skyrmions via a pure thermal effect 19-21 has not been experimentally demonstrated so far; moreover, whether the skyrmion motion driven by thermal gradients follows the direction of thermal diffusion or, oppositely, the direction of magnonic spin torque 15,20,22,23 remains an open question. approach allows us to study the dynamics of skyrmions induced by a perpendicular magnetic field (μ 0 H ⊥), electrical current (j e), temperature (T) and temperature gradient (ΔT(x)). The magnetic imaging was conducted at the Fe L 3 edge Q6
Artificial synapses can boost neuromorphic computing to overcome the inherent limitations of von Neumann architecture. As a promising memristor candidate, ferroelectric tunnel junctions (FTJ) enable the authors to successfully emulate spike-timing-dependent synapses. However, the nonlinear and asymmetric synaptic weight update under repeated presynaptic stimulation hampers neuromorphic computing by favoring the runaway of synaptic weights during learning. Here, the authors demonstrate an FTJ whose conductivity varies linearly and symmetrically by judiciously combining ferroelectric domain switching and oxygen vacancy migration. The artificial neural network based on this FTJ-synapse achieves classification accuracy of 96.7% during supervised learning, which is the closest to the maximum theoretical value of 98% achieved to date. This artificial synapse also demonstrates stable unsupervised learning in a noisy environment for its well-balanced spike-timing-dependent plasticity response. The novel concept of controlling ionic migration in ferroelectric materials paves the way toward highly reliable and reproducible supervised and unsupervised learning strategies.
Spintronic devices are considered a possible solution for the hardware implementation of artificial synapses and neurons, as a result of their non-volatility, high scalability, complementary metal-oxide-semiconductor transistor compatibility, and low power consumption. As compared to ferromagnets, ferrimagnet-based spintronics exhibits equivalently fascinating properties that have been witnessed in ultrafast spin dynamics, together with efficient electrical or optical manipulation. Their applications in neuromorphic computing, however, have still not been revealed, which motivates the present experimental study. Here, by using compensated ferrimagnets containing Co 0.80 Gd 0.20 with perpendicular magnetic anisotropy, it is demonstrated that the behavior of spin-orbit torque switching in compensated ferrimagnets could be used to mimic biological synapses and neurons. In particular, by using the anomalous Hall effect and magneto-optical Kerr effect imaging measurements, the ultrafast stimulation of artificial synapses and neurons is illustrated, with a time scale down to 10 ns. Using experimentally derived device parameters, a threelayer fully connected neural network for handwritten digits recognition is further simulated, based on which, an accuracy of more than 93% could be achieved. The results identify compensated ferrimagnets as an intriguing candidate for the ultrafast neuromorphic spintronics.
The discovery of magnetic skyrmions provides a promising pathway for developing functional spintronic memory and logic devices. Towards the future high-density memory application, nanoscale skyrmions with miniaturized diameters, ideally down to 20 nm are required. Using x-ray magnetic circular dichroism transmission microscopy, nanoscale skyrmions are observed in the [Pt/Co/Ir]15 multilayer at room temperature. In particular, small skyrmions with minimum diameters approaching 20 nm could be generated by the current-induced spin-orbit torques. Through implementing material specific parameters, the dynamic process of skyrmion generation is further investigated by performing micromagnetic simulations. According to the simulation results, we find that both the tube-like Néel-type skyrmions and the bobber-like Néel-type skyrmions can be electrically generated. In particular, the size of the bobber-like Néel-type skyrmions can be effectively reduced by the spin-orbit torques, which leads to the formation of 20 nm Néel-type skyrmions. Our findings could be important for understanding the formation dynamics of nanoscale Néel-type spin textures, skyrmions and bobber in particular, which could also be useful for promoting nanoscale skyrmionic memories and logic devices.
Van der Waals (vdW) ferromagnetic materials have attracted considerable attention in the nanomaterial community, which could provide a unique platform to study magnetism at the nanoscale. Along this direction, many interesting results have been reported, including the electric field control of magnetism and topological spin textures. In this report, we present a rapid and spatially resolved imaging method to study the dimensionality-dependent magnetic properties of Fe3GeTe2 (FGT) nanoflakes. Our method is named as polar magneto-optical Kerr imaging microscopy magnetometry (p-MIMM), which is made possible by analyzing the intensity evolution of wide-field polar magneto-optical Kerr effect (MOKE) images that were collected by varying magnetic fields, thicknesses, and temperatures. In particular, spatially resolved MOKE hysteresis loops can be acquired in the FGT nanoflakes with a submicrometer resolution. By analyzing the evolution of the relative (saturated) MOKE intensity as a function of temperature, we further study the critical exponent and universality class and its dependence on the FGT nanoflake thickness. Combining the polar MOKE images with the calculated MOKE hysteresis loops, a detailed magnetic phase diagram summarizing an evolution of the stripe domain, single domain, and paramagnetic state is further validated. Our results suggest that the wide-field p-MIMM can be conveniently used for rapidly examining the magnetic properties of versatile vdW magnetic materials.
Rechargeable lithium batteries are the most practical and widely used power sources for portable and mobile devices in modern society. Manipulation of the electronic and ionic charge transport and accumulation in solid materials has always been crucial for rechargeable lithium batteries. The transport and accumulation of lithium ions in electrode materials, which is a diffusion process, is determined by the concentration distribution of lithium ions and the intrinsic structure of the electrode material and thus far has not been manipulated by an external force. Here, we report the realization of controllable two-dimensional movement and redistribution of lithium ions in metal oxides. This achievement is one kind of centimeter-scale control and is achieved by a magnetic field based on the ‘current-driving model’. This work provides additional insight for building safe and high-capacity rechargeable lithium batteries.
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