We theoretically investigate dark dimer mode excitation and strong coupling with a nanorod dipole. Efficient excitation of a dark mode in a gold (Au) nanorod dimer using an electric dipole can be achieved by an optimal overlap between the dipole moment and dark modal field. By replacing the dipole emitter with an Au nanorod, a plane wave excited dipole mode in the nanorod can be effectively coupled to the dark dimer mode through nearfield interaction. At a 10-nm separation of the nanorod and the dimer, plasmonic interaction between dipole-dark modes enters the strong coupling regime with a Rabi-like splitting of 219.2 meV, which is further evidenced by the anticrossing feature and Rabi-like oscillation of electromagnetic energy of the coupled modes. Our results propose an efficient approach to far-field activating dark modes in coupled nanorod dimers and exchanging plasmonic excitations at nanoscale, which may open new opportunities for nanoplasmonic applications such as nanolasers or nanosensors.
Chiral structures are promising in many applications, such as biological sensing and analytical chemistry, and have been extensively explored. In this paper, we theoretically investigate the chiral response of twisted bilayer α-MoO3. Firstly, the analytical formula for the transmissivity is derived when the structure is illuminated with circularly polarized plane waves. Furthermore, the results demonstrate that the twisted bilayer α-MoO3 can excite the strong chirality with the maximum circular dichroism (CD) of 0.89. In this case, the chirality is due to the simultaneous breaking the rotational symmetry and mirror symmetry, which originates from the relative rotation of two α-MoO3 layers. To better understand the physical mechanism, the polarization conversion between the left-hand circular polarization (LCP) and right-hand circular polarization (RCP) waves is discussed as well. Moreover, it is found that the structure can maintain the strong chirality (CD > 0.8) when the twisted angle varies from 69° to 80°, which effectively reduces the strictness in the requirement for rotation angle. In addition, the CD can be larger than 0.85 when the incidence angle of circularly polarized plane wave is less than 40°, implying that the chirality is robust against the angle of incidence. Our work not only provides an insight into chirality induced by the twisted bilayer α-MoO3, but also looks forward to applications in biological sensing.
The ability to sense heat and touch is essential for healthcare, robotics, and human–machine interfaces. By taking advantage of the engineerable waveguiding properties, we design and fabricate a flexible optical microfiber sensor for simultaneous temperature and pressure measurement based on theoretical calculation. The sensor exhibits a high temperature sensitivity of 1.2 nm/°C by measuring the shift of a high-order mode cutoff wavelength in the short-wavelength range. In the case of pressure sensing, the sensor shows a sensitivity of 4.5% per kilopascal with a fast temporal frequency response of 1000 Hz owing to the strong evanescent wave guided outside the microfiber. The cross talk is negligible because the temperature and pressure signals are measured at different wavelengths based on different mechanisms. The properties of fast temporal response, high temperature, and pressure sensitivity enable the sensor for real-time skin temperature and wrist pulse measurements, which is critical to the accurate analysis of pulse waveforms. We believe the sensor will have great potential in wearable optical devices ranging from healthcare to humanoid robots.
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By placing a single Au nanoparticle on the surface of a cadmium sulfide (CdS) nanowire, we demonstrate strong coupling of localized surface plasmon resonance (LSPR) modes in the nanoparticle and whispering gallery modes (WGMs) in the nanowire. For a 50-nm-diameter Au-nanosphere particle, strong coupling occurs when the nanowire diameter is between 300 and 600 nm, with a mode splitting up to 80 meV. Using a temperature-induced spectral shift of the resonance wavelength, we also observe the anticrossing behavior in the strongly coupled system. In addition, since the Au nanosphere has spherical symmetry, the supported LSPR mode can be selectively coupled with transverse electric (TE) and transverse magnetic (TM) WGMs in the nanowire. The ultracompact strong-coupling system shown here may provide a versatile platform for studying hybrid “photon–plasmon” nanolasers, nonlinear optical devices, and nanosensors.
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