Electrochromic materials are widely used in smart windows. An ideal future electrochromic window would be able to control visible light transmission, tune building's heat conversion of near-infrared (NIR) solar radiation, and reduce attacks by microorganisms. To date, most of the reports have primarily focused on visible-light transmission modulation using electrochromic materials. Herein, we report the fabrication of an electrochromic-photothermal film by integrating electrochromic WO with plasmonic Au nanostructures and demonstrate its adjustability during optical transmission and photothermal conversion of visible and NIR lights. The localized surface plasmon resonance (LSPR) of Au nanostructures and the broadband nonradiative plasmon decay are proposed to be tunable using both the electric field and the WO substrate. Further enhanced photothermal conversion is achieved in colored state, which is attributed to coupling of traditional visible-band optical switching with NIR-LSPR extinction. The resulted electrochromic-photothermal film can also effectively reduce the numbers of attacking microorganisms, thus promising for use as a sterile smart window for advanced applications.
Modern nanophotonic and meta-optical devices utilize a tremendous number of structural degrees of freedom to enhance light–matter interactions. A fundamental question is how large such enhancements can be. We develop an analytical framework to derive upper bounds to single-frequency electromagnetic response, across near- and far-field regimes, for any materials, naturally incorporating the tandem effects of material- and radiation-induced losses. Our framework relies on a power-conservation law for the polarization fields induced in any scatterer. It unifies previous theories on optical scattering bounds and reveals new insight for optimal nanophotonic design, with applications including far-field scattering, near-field local-density-of-states engineering, optimal wavefront shaping, and the design of perfect absorbers. Our bounds predict strikingly large minimal thicknesses for arbitrarily patterned perfect absorbers, ranging from 50–100 nm for typical materials at visible wavelengths to micrometer-scale thicknesses for polar dielectrics at infrared wavelengths. We use inverse design to discover metasurface structures approaching the minimum-thickness perfect-absorber bounds.
We demonstrate technological improvements in phonon sector tests of the Lorentz invariance that implement quartz bulk acoustic wave oscillators. In this experiment, room temperature oscillators with state-of-the-art phase noise are continuously compared on a platform that rotates at a rate of order of a cycle per second. The discussion is focused on improvements in noise measurement techniques, data acquisition, and data processing. Preliminary results of the second generation of such tests are given, and indicate that standard model extension coefficients in the matter sector can be measured at a precision of order 10 GeV after taking a year's worth of data. This is equivalent to an improvement of two orders of magnitude over the prior acoustic phonon sector experiment.
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