The rapid development of electronic skins has allowed novel multifunctional human–machine interaction interfaces, especially in motion interaction sensors. Although motion sensing is widely used in advanced flexible electronic devices through the integration of single sensing units, the number of electrodes has increased with the increase in integration by the square multiple. This paper presents a self‐powered electronic skin based on the Archimedes spiral structure design, which can detect the multi‐directional movement of the slider without external energy supply. As the rotation angle of the Archimedes spiral increases from 2π to 4π, the maximum resolvable movement direction of the device increases from 24 to 280, and the number of electrodes is kept at 4. Through the exploration of the principle of triboelectricity, the inherent electronegativity of the triboelectric materials is used as the basis for signal discrimination, which not only increases the reliability of the device, but also solves the problem of energy supply during device operation. A reduced number of electrodes and its battery‐free nature enables this electronic skin to be easily integrated into portable electronic devices, such as laptops, smart phones, healthcare devices, etc.

Multifunctional sensing systems play important roles in a variety of applications, incluing health surveillance, intelligent prothetics, human–machine/ambinece interfaces, and many others. The richness of the signal and the decoupling among multiple parameters are essential for simultaneous, multimodal measurements. However, current multifunctional sensing fails to decouple interferences from various signals. Here, we propose a double-sided wearable system that both enables multifunctional sensing and avoids the interferences among multiple parameters. Specifically, the sensitivities of system modules to strain are controlled through customizing the pattern and morphology of sensing electrodes as well as the modification of active materials. Compensation of temperature drift and selection of sensing mechanisms ensure the thermal stability of the system. The encapsulation of modules resists the interferences of proximity, normal pressure, and gas molecules at the same time. A double-sided partition layout with serpentine interconnections reduces the effect of motion artifacts and ensures simultaneous operation of electrochemical-sensing modules. Cooperation among decoupled modules acts as the bridge between the perception of ambience changes and the timely feedback of the human body. In addition, to sense the signal at the interface, modules for energy harvesting and storage are also integrated into the system to broaden its application scenarios.

rigid devices, soft microsystems commonly adopt functional materials with appealing properties, such as dielectric elastomers, [10] shape-memory polymers, [11] liquid metals, [12] and hydrogels. [13] Reliable actuation is of vital importance in micro systems, especially for energy harvesting, where the mechanical stability, controllability, and adaptability are highly desired to maintain the long-term power output in a complex environment. Recent advances in materials have enabled soft actuators with different driving mechanisms, including magnetic effect, [14] chemical effect, [15] photo thermal effect, [16] and electrical effect. [17] The introduction of biomimetic designs or multidimensional geometries allows for the continuous operation in complex environments. [18][19][20][21][22] Among these strategies, the magnetic-controlled approach shows compelling advantages, due to its fast response, large deformation, precise control and stable repeatability. [23][24][25] Magnetic materials deform under external magnetic fields, which is crucial for magnetic-controlled structures. [26][27][28] Most magnetic-controlled robotics exploit magnetic materials to achieve various locomotion, where the permanent and programmed magnetization profiles are key design parameters. [29] Strong magnetic fields from these permanent magnets pose a variety of incompatibility issues in scenarios such as electronic circuit, biomedicine, and micro/nanomanufacturing. By contrast, magneticThe advent of functional materials offers tremendous potential in a broad variety of areas such as electronics, robotics, and energy devices. Magnetic materials are an attractive candidate that enable multifunctional devices with capabilities in both sensing and actuation. However, current magnetic devices, especially those with complex motion modalities, rely on permanently magnetized materials with complicated, non-uniform magnetization profiles. Here, based on magnetic materials with temporary-magnetization, a mechanically guided assembly process successfully converts laser-patterned 2D magnetic materials into judiciously engineered 3D structures, with dimensions and geometries ranging from mesoscale 3D filaments, to arrayed centimeter-scale 3D membranes. With tailorable mechanical properties and highly adjustable geometries, 3D soft structures can exhibit various tethered locomotions under the precise control of magnetic fields, including local deformation, unidirectional tilting, and omnidirectional rotation, and can serve as dynamic surfaces for further integration with other functional materials or devices. Examples demonstrated here focus on energy-harvesting systems, including 3D piezoelectric devices for noncontact conversion of mechanical energy and active motion sensing, as well as 3D solar tracking systems. The design strategy and resulting magnetic-controlled 3D soft structures hold great promise not only for enhanced energy harvesting, but also for multimodal sensing, robotic interfaces, and biomedical devices.

Graphene‐based phosphorus‐doped carbon (GPC) is prepared through a facile and scalable thermal annealing method by triphenylphosphine and graphite oxide as precursor. The P atoms are successfully doped into few layer graphene with two forms of P–O and P–C bands. The GPC used as anode material for Na‐ion batteries delivers a high charge capacity 284.8 mAh g−1 at a current density of 50 mA g−1 after 60 cycles. Superior cycling performance is also shown at high charge−discharge rate: a stable charge capacity 145.6 mAh g−1 can be achieved at the current density of 500 mA g−1 after 600 cycles. The result demonstrates that the GPC electrode exhibits good electrochemical performance (higher reversible charge capacity, super rate capability, and long‐term cycling stability). The excellent electrochemical performance originated from the large interlayer distance, large amount of defects, vacancies, and active site caused by P atoms doping. The relationship of P atoms doping amount with the Na storage properties is also discussed. This superior sodium storage performance of GPC makes it as a promising alternative anode material for sodium‐ion batteries.