Streamer properties such as their velocity, diameter, intensity and density, can be obtained by analysis of temporal and spatial resolved ICCD imaging. In this paper, experimental results on streamer generation and propagation as a function of several high-voltage pulse and reactor parameters are described. Experiments were performed on a large scale wire–plate reactor in ambient air. The set-up allows for independent variation of the parameters over wide ranges. The minimum gate time of the ICCD camera is 5 ns, allowing for a high temporal resolution. The camera can be triggered with a precision of 1 ns. Both negative and positive polarity pulses are investigated. The most important conclusions are as follows. (1) The streamer velocity ((0.5–2.5) × 106 m s−1) increases if the applied electric field and/or the voltage rise rate is increased. (2) The same is true regarding the velocity ((0.2–1.2) × 105 m s−1) with which the streamer diameter (0.7–3.0 mm) increases during propagation. (3) Typical properties (velocity, diameter, etc) of negative and positive polarity streamers vary less than 25%, especially when the applied electric field is high. (4) As long as the dc bias voltage is below the dc corona onset value it does not have a separate effect on the visual streamer properties. Only the total voltage (peak voltage + dc) is of importance. (5) A simple model was used to determine the electric field in the secondary streamer channel. It was found that in the light emitting part of the secondary streamer the electric field is approximately 21.5 kV cm−1. In the remainder (dark part) of the channel the electric field is around 6.5 kV cm−1. This paper shows mainly experimental findings. Not all observed relations and phenomena could be explained. This is partly caused by the fact that current theoretical and numerical models are not yet able to describe the experimental situation as used during this study.
In this paper a large-scale pulsed corona system is described in which pulse parameters such as pulse rise-time, peak voltage, pulse width and energy per pulse can be varied. The chemical efficiency of the system is determined by measuring ozone production. The temporal and spatial development of the discharge streamers is recorded using an ICCD camera with a shortest exposure time of 5 ns. The camera can be triggered at any moment starting from the time the voltage pulse arrives on the reactor, with an accuracy of less than 1 ns. Measurements were performed on an industrial size wire-plate reactor. The influence of pulse parameters like pulse voltage, DC bias voltage, rise-time and pulse repetition rate on plasma generation was monitored. It was observed that for higher peak voltages, an increase could be seen in the primary streamer velocity, the growth of the primary streamer diameter, the light intensity and the number of streamers per unit length of corona wire. No significant separate influence of DC bias voltage level was observed as long as the total reactor voltage (pulse + DC bias) remained constant and the DC bias voltage remained below the DC corona onset. For those situations in which the plasma appearance changed (e.g. different streamer velocity, diameter, intensity), a change in ozone production was also observed. The best chemical yields were obtained for low voltage (55 kV), low energetic pulses (0.4 J/pulse): 60 g (kWh)−1. For high voltage (86 kV), high energetic pulses (2.3 J/pulse) the yield decreased to approximately 45 g (kWh)−1, still a high value for ozone production in ambient air (RH 42%). The pulse repetition rate has no influence on plasma generation and on chemical efficiency up to 400 pulses per second.
This paper presents a circuit topology to obtain current multiplication by using multiple thyristors. To gain insight into this technique, an equivalent circuit model is introduced. Proper operation of the topology was demonstrated by experiments on a small-scale setup including three thyristors. One thyristor is triggered by a trigger circuit; the other two are autotriggered and require no external trigger circuit. The three thyristors could be synchronized automatically in sequence. During the closing process, the discharging of the energy storage capacitors via the thyristors is prevented. The discharging starts when all thyristors are closed, and the currents through each thyristor are simultaneous and identical. The output current is exactly three times the switching current.
Gas cleaning using plasma technology is slowly introduced into industry nowadays. Several challenges still have to be overcome: increasing the scale, safety, life-time and reducing costs. In 2006 we demonstrated a 20 kW nanosecond pulsed corona system. The electrical efficiency was > 90%. O-radical yields were found to be very high (3-7 mole/kWh). However, to be competitive, high costs of the pulsed power technology are still a major hurdle. Here we present a novel modulator for efficient generation of large volume corona plasma. Only a small amount of expensive high-voltage components are required. Switching is done at an intermediate voltage level of 1 kV with standard thyristors. At the high-voltage side, only a diode and a pulse transformer are needed. The estimated costs are about 5 kEuro/kW, whereas for state-of-the-art pulsed power technology these costs usually are about 20-30 kEuro/kW. Detailed investigations on the modulator and a wire-plate corona reactor will be presented. Modulator parameters have been varied systematically as well as reactor parameters (number of electrodes, electrode-plate distance). The O-radical yield was determined from the measured ozone concentrations at the exhaust of the reactor. With a detailed kinetic model, ozone concentrations could be calculated back to the initial O*-yields. The following conclusions will be discussed: for all parameters, an electrical efficiency of > 90% could be obtained. With fast imaging, the average streamer width was found to be ∼ 737 µm and an estimate for the plasma volume was made. The obtained yields of O-radicals (1-4 mole/kWh) are excellent. The conditions to obtain high yields will be discussed.
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