We perform a systematic analysis of the influence of phonon driving on the superconducting Holstein model coupled to heat baths by studying both the transient dynamics and the nonequilibrium steady state (NESS) in the weak and strong electron-phonon coupling regimes. Our study is based on the nonequilibrium dynamical mean-field theory, and for the NESS we present a Floquet formulation adapted to electron-phonon systems. The analysis of the phonon propagator suggests that the effective attractive interaction can be strongly enhanced in a parametric resonant regime because of the Floquet side bands of phonons. While this may be expected to enhance the superconductivity (SC), our fully self-consistent calculations, which include the effects of heating and nonthermal distributions, show that the parametric phonon driving generically results in a suppression or complete melting of the SC order. In the strong coupling regime, the NESS always shows a suppression of the SC gap, the SC order parameter, and the superfluid density as a result of the driving, and this tendency is most prominent at the parametric resonance. Using the real-time nonequilibrium DMFT formalism, we also study the dynamics towards the NESS, which shows that the heating effect dominates the transient dynamics, and SC is weakened by the external driving, in particular at the parametric resonance. In the weak coupling regime, we find that the SC fluctuations above the transition temperature are generally weakened under the driving. The strongest suppression occurs again around the parametric resonances because of the efficient energy absorption.
We study the dynamics of excitonic insulators coupled to phonons using the time-dependent mean-field theory. Without phonon couplings, the linear response is given by the damped amplitude oscillations of the order parameter with a frequency equal to the minimum band gap. A phonon coupling to the interband transfer integral induces two types of long-lived collective oscillations of the amplitude, one originating from the phonon dynamics and the other from the phase mode, which becomes massive. We show that, even for small phonon coupling, a photoinduced enhancement of the exciton condensation and the gap can be realized. Using the Anderson pseudospin picture, we argue that the origin of the enhancement is a cooperative effect of the massive phase mode and the Hartree shift induced by the photoexcitation. We also discuss how the enhancement of the order and the collective modes can be observed with time-resolved photoemission spectroscopy. [7][8][9][10][11][12]. An EI state is formed by the macroscopic condensation of electron-hole pairs [13,14], and its theoretical description is analogous to the BCS or Bose-Einstein condensate (BEC) theory for SC. Although the idea of exciton condensation was proposed already in the 1960s [13][14][15], the interest in this topic has been renewed recently by the study of some candidate materials such as 1T-TiSe 2 and Ta 2 NiSe 5 (TNS) [16][17][18][19][20][21]. Their analogy to SC makes the EI an interesting system for nonequilibrium studies. In particular, for TNS, time-and angle-resolved photoemission spectroscopy (trARPES) experiments showed that the direct band gap can be either decreased or increased depending on the pump fluence [11], which was interpreted in terms of a photoinduced enhancement or suppression of excitonic order. A more recent report of the amplitude mode [12] provides further confirmation of an EI state in TNS.So far, the theoretical works on EIs have mainly focused on the equilibrium properties such as the BEC-BCS crossover [22,23], the coupling of the EI to phonons [24][25][26], linear susceptibilities [27][28][29], and the effect of strong interactions and new emergent phases [30][31][32]. In contrast, the nonequilibrium investigation of EIs has just begun [10]. In this work, using TNS as a model system, we clarify two basic effects of the electron-phonon (e-ph) coupling on the dynamics of EIs: (i) the effect on collective modes and (ii) the impact on the excitonic order after
Using Floquet dynamical mean-field theory, we study the high-harmonic generation in the time-periodic steady states of wide-gap Mott insulators under ac driving. In the strong-field regime, the harmonic intensity exhibits multiple plateaus, whose cutoff energies ε_{cut}=U+mE_{0} scale with the Coulomb interaction U and the maximum field strength E_{0}. In this regime, the created doublons and holons are localized because of the strong field and the mth plateau originates from the recombination of mth nearest-neighbor doublon-holon pairs. In the weak-field regime, there is only a single plateau in the intensity, which originates from the recombination of itinerant doublons and holons. Here, ε_{cut}=Δ_{gap}+αE_{0}, with Δ_{gap} the band gap and α>1. We demonstrate that the Mott insulator shows a stronger high-harmonic intensity than a semiconductor model with the same dispersion as the Mott insulator, even if the semiconductor bands are broadened by impurity scattering to mimic the incoherent scattering in the Mott insulator.
We study the relaxation of the Holstein model after a sudden switch-on of the interaction by means of the nonequilibrium dynamical mean field theory, with the self-consistent Migdal approximation as an impurity solver. We show that there exists a qualitative change in the thermalization dynamics as the interaction is varied in the weak-coupling regime. On the weaker interaction side of this crossover, the phonon oscillations are damped more rapidly than the electron thermalization timescale, as determined from the relaxation of the electron momentum distribution function. On the stronger interaction side, the relaxation of the electrons becomes faster than the phonon damping. In this regime, despite long-lived phonon oscillations, a thermalized momentum distribution is realized temporarily. The origin of the "thermalization crossover" found here is traced back to different behaviors of the electron and phonon self-energies as a function of the electron-phonon coupling. In addition, the importance of the phonon dynamics is demonstrated by comparing the self-consistent Migdal results with those obtained with a simpler Hatree-Fock impurity solver that neglects the phonon self-energy. The latter scheme does not properly describe the evolution and thermalization of isolated electron-phonon systems.
We study collective amplitude modes of the superconducting order parameter in strongly coupled electronphonon systems described by the Holstein model using the nonequilibrium dynamical mean-field theory with the self-consistent Migdal approximation as an impurity solver. The frequency of the Higgs amplitude mode is found to coincide with the superconducting gap even in the strongly coupled (beyond BCS) regime. Besides the Higgs mode, we find another collective mode involving the dynamics of both the phonons and the superconducting order parameter. The frequency of this mode, higher than twice the renormalized phonon frequency in the superconducting phase, is shown to reflect a strong electron-mediated phonon-phonon interaction. Both of collective modes are predicted to contribute to time-resolved photoemission spectra after a strong laser pump as vertex corrections to produce resonance peaks, which allows one to distinguish them from quasiparticle excitations.
Strongly correlated electron systems; heavy fermions PACS 71.10.Fd -Lattice fermion models (Hubbard model, etc.)Abstract. -We demonstrate the existence of long-lived prethermalized states in the Mott insulating Hubbard model driven by periodic electric fields. These states, which also exist in the resonantly driven case with a large density of photo-induced doublons and holons, are characterized by a nonzero current and an effective temperature of the doublons and holons which depends sensitively on the driving condition. Focusing on the specific case of resonantly driven models whose effective time-independent Hamiltonian in the high-frequency driving limit corresponds to noninteracting fermions, we show that the time evolution of the double occupation can be reproduced by the effective Hamiltonian, and that the prethermalization plateaus at finite driving frequency are controlled by the next-to-leading order correction in the high-frequency expansion of the effective Hamiltonian. We propose a numerical procedure to determine an effective Hubbard interaction that mimics the correlation effects induced by these higher order terms.
We study the Holstein-Hubbard model at half filling to explore ordered phases including superconductivity (SC), antiferromagnetism (AF), and charge order (CO) in situations where the electron-electron and electron-phonon interactions are strong (∼ electronic bandwidth). The model is solved in the dynamical mean-field approximation using a continuous-time quantum Monte Carlo impurity solver. We determine the superconducting transition temperature (Tc) and the SC order parameter and show that the phonon-induced retardation or the strong Coulomb interaction leads to a significant reduction and shift of the Tc dome if one interprets the system as having an effective static interaction U eff given by the Hubbard U reduced by the phonon-mediated attraction in the static limit. This behavior is analyzed by comparison to an effective static model in the polaron representation with a reduced bandwidth. We also determine the finite-temperature phase diagram including AF and CO. In the moderate-coupling regime, there is a hysteretic region of AF and CO around U eff = 0, while the two phases are separated by a paramagnetic metal in the weak-coupling regime and a paramagnetic insulator in the strong coupling regime.
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