A comprehensive review of Pt electrocatalysts for the oxygen reduction reaction: nanostructure, activity, mechanism and carbon support in PEM fuel cells. Journal of Materials Chemistry A, 5 (5). pp. 1808 -1825 . ISSN 2050 Access from the University of Nottingham repository: http://eprints.nottingham.ac.uk/40957/1/Journal%20of%20Materials%20Chemistry%20A %EF%BC%88C6TA08580F%20-%20corrected%20proofs%20-final%EF%BC%89.pdf
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A note on versions:The version presented here may differ from the published version or from the version of record. If you wish to cite this item you are advised to consult the publisher's version. Please see the repository url above for details on accessing the published version and note that access may require a subscription. Translation errors between word-processor files and typesetting systems can occur so the whole proof needs to be read. Please pay particular attention to: tabulated material; equations; numerical data; figures and graphics; and references. If you have not already indicated the corresponding author(s) please mark their name(s) with an asterisk. Please e-mail a list of corrections or the PDF with electronic notes attached -do not change the text within the PDF file or send a revised manuscript. Corrections at this stage should be minor and not involve extensive changes. All corrections must be sent at the same time.Please bear in mind that minor layout improvements, e.g. in line breaking, table widths and graphic placement, are routinely applied to the final version.We will publish articles on the web as soon as possible after receiving your corrections; n no late corrections will be made. The sluggish rate of the oxygen reduction reaction (ORR) in proton exchange membrane (PEM) fuel cells has been a major challenge. Significantly increasing efforts have been made worldwide towards a highly active ORR catalyst with high durability. Among all the catalysts exploited, Pt electrocatalysts are still the best in terms of a comprehensive evaluation. The investigation of Pt-based ORR catalysts is necessary for a practical ORR catalyst with low Pt content. This paper reviews recent progress in the studies of the mechanism, nanostructure, size effect and carbon supports of Pt electrocatalysts for the ORR. The importance of the size and structure control of Pt ORR catalysts, related with carbon support materials, is indicated. The potential methods for such control are discussed. The progress in theoretical studies and in situ catalyst characterization are also discussed. Finally, challenges and future developments are addressed.
Due to their low cost, light weight and corrosive resistant features, polymer heat exchangers have been intensively studied by researchers with the aim to replace metallic heat exchangers in a wide range of applications. This paper reviews the development of polymer heat exchangers in the last decade, including cutting edge materials characteristics, heat transfer enhancement methods of polymer materials and a wide range of polymer heat exchanger applications. Theoretical modelling and experimental testing results have been reviewed and compared with literature. A recent development, the polymer micro-hollow fibre heat exchanger, is introduced and described. It is shown that polymer materials do hold promise for use in the construction of heat exchangers in many applications, but that a considerable amount of research is still required into material properties, thermal performance and life-time behaviour.
Highlights 1. Polysaccharide-based aerogels can be prepared with supercritical or freeze drying. 2. Polysaccharide-based aerogels may have nm-μm pore size distribution. 3. Aerogels with open or close pores have different functions and applications. 4. The formula and drying methods can change the pore structure and functions. 5. Advances and future challenges of polysaccharide-based aerogels are clarified. Highlights (for review)
In the history, architecture was exploited to the human being to protect him from unsteady environmental conditions. In the past centuries, architecture was pioneer art which has special features such as; simplicity, organization, clear style, accurate decoration, material assembly, and so on. However, modern buildings become complex products that have so many parts which have to fulfil different functions. Therefore, new computational ways and techniques have been developed to facilitate the design of modern complicated buildings and to create a convenient quantitative relationship between the environment and the envelope, putting into consideration the obstacles which influence on the building design. This has therefore formed the concept of parametric design in architecture, in order to deal with complex designs and gain more accurate results. Modern architects claim that parametric design is the most creative way to understand the development and complexity of the new era of architectural trends [1]. Meanwhile, it is really hard to deal with sophisticated details in buildings using our brains to imagine, or conventional ways to design [2]. In addition, building technologies nowadays are integrated and containing many disciplines in the same time, and each discipline is dependent on the other disciplines in a very complex vast connections. Hence, they should be organized in a database container, and this container could be managed parametrically using parametric design as an advanced way to explore and understand these sophisticated relations [3]. This paper hence presents a literature review on parametric design in architecture practice and put a focus on its applications in daylighting and solar radiation, which can have an essential impact on improving daylight availability and energy saving.
Compound parabolic concentrator (CPC) has been gaining ever-increasing attention from academic researchers and industrial developers owing to its stationary feature for solar energy collection with a higher efficiency. As a low concentration concentrator with a larger acceptance angle and without a tracking requirement, it is an attractive solution to improve the system performance and reduce the cost of photovoltaic (PV) system, solar thermal system, daylighting and lighting systems, etc. This study will present a comprehensive and up-to-date review of its design principles for miscellaneous configurations, applications, performance predictions and technological advances. Numerous technically focused studies since 2000 will be introduced and summarized. Finally, the outlook focusing on CPC designs and improvements will be proposed.
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