Central Asia is one of the most important sources of mineral saline dust worldwide. A comprehensive understanding of Central Asian dust transport is essential for evaluating its impacts on human health, ecological safety, weather and climate. This study first puts forward an observation-based climatology of Central Asian dust transport flux by using the 3-D dust detection of Cloud-Aerosol LiDAR with Orthogonal Polarization (CALIOP). The seasonal difference of transport flux and downstream contribution are evaluated and compared with those of the Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2). Central Asian dust can be transported not only southward in summer under the effect of the South Asian summer monsoon, but also eastward in other seasons under the control of the westerly jet. Additionally, the transport of Central Asian dust across the Pamir Plateau to the Tibetan Plateau is also non-negligible, especially during spring (with a transport flux rate of 150 kg m−1 day−1). The annual CALIOP-based downstream contribution of Central Asian dust to South Asian (164.01 Tg) is 2.1 times that to East Asia (78.36 Tg). This can be attributed to the blocking effect of the higher terrain between Central and East Asia. Additionally, the downstream contributions to South and East Asia from MERRA-2 are only 0.36 and 0.84 times that of CALIOP, respectively. This difference implies the overestimation of the wet and dry depositions of the model, especially in the low latitude zone. The quantification of the Central Asian dust transport allows a better understanding of the Central Asian dust cycle, and supports the calibration/validation of aerosol-related modules of regional and global climate models.
Monodisperse Mn3O4 nanoparticles were prepared solvothermally starting from manganese acetate by using polyether amide block copolymers (Pebax2533) as a template in isopropanol. The diameter of the nanoparticles in the range of 8.7 nm∼31.5 nm was decreased with increase of Pebax2533 concentration. The electrochemical properties and application in supercapacitor of Mn3O4 nanoparticles were further studied. The results showed that smaller nanoparticles had a larger capacitance. The higher capacitance of 217.5 F/g at a current density of 0.5 A/g was obtained on 8.7 nm Mn3O4 nanoparticles. The specific capacitance retention of 82% was maintained after 500 times of continuous charge-discharge cycles.
Summer dust aerosol in the Taklimakan Desert (TD) affects not only the albedo of the snow and ice sheets on the Tibetan Plateau (TP) but also air quality and precipitation in the downstream areas. In this study, the summer extreme dust activity in the TD was jointly investigated by using satellite observations and MERRA-2 reanalysis datasets and divided into two states: dust active period and dust inactive period. The horizontal and vertical distribution of summer dust during both the dust active and inactive periods, as derived from the MERRA-2 dataset, is consistent with satellite observations. By comparing the upper-level circulation and surface meteorological elements at two periods, we identify the South Asian High (SAH) as the dominant factor driving the extreme dust activity in the TD during summer. When the SAH is centered on the Iranian Plateau (IP), the dust aerosol in the TD exhibits increased activity and is lifted to higher altitudes due to significantly enhanced westerly winds, near-surface wind speed, and an ascending motion. Conversely, when the SAH is centered on the TP, the summer dust activity shows the opposite behavior. These new findings on the regulatory mechanism of the SAH on the summer dust activity in the TD are highly significant for understanding the occurrence and transport of summer Asian dust and its potential impact on heavy precipitation in the downstream areas.
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