A novel approach has been proposed for improving the performance of lithium-sulfur batteries (LSBs) with a carbon-based material as an interlayer between the cathode and separator. With this method, the cross-over of lithium polysulfides (LiPS) to the anode is suppressed, increasing reutilization of the sulfur cathode. In this study, activated carbons (ACs) were prepared using coffee waste as a carbon source and potassium hydroxide (KOH) as an activation agent at various reaction temperatures ranging from 500 to 800 °C. With the rise in heating temperature, the specific surface areas, micro-surface areas, and micro-pore volumes of the AC samples gradually increased. In particular, the AC sample prepared at 800 °C and used as a functional separator for LSB exhibited improved capacity and cycling performance while suppressing the LiPS shuttle effect.
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