Challenging precious Pt-based electrocatalysts for dye-sensitized solar cells (DSSCs), graphene nanoplatelets that are N-doped at the edges (NGnPs) are prepared via simply ball-milling graphite in the presence of nitrogen gas. DSSCs based on specific nanoplatelets designated "NGnP5" display superior photovoltaic performance (power conversion efficiency, 10.27%) compared to that of conventional Pt-based devices (9.96%). More importantly, the NGnP counter electrode exhibits outstanding electrochemical stability and electrocatalytic activity with a cobalt-complex redox couple.
Edge-carboxylated graphene nanoplatelets (ECGnPs) prepared by the dry ball-milling of graphite showed lower charge-transfer resistance (RCT) and better electrochemical stability for the JK-303-based solar cell with Co(bpy)32+/3+ redox couple.
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