We fabricated quasiantiferromagnetic (quasi-AFM) layers with alternating antiparallel magnetization in the neighboring domains via 90° magnetic coupling through an Fe-O layer. We investigated the magnetic properties and the relationship between the magnetic domain size and the 90° magnetic coupling via experiments and calculations. Two types of samples with a Ru buffer and a (Ni80Fe20)Cr40 buffer were prepared, and we found that with the NiFeCr buffer, the sample has a flatter Fe-O layer, leading to stronger 90° magnetic coupling and a smaller domain size compared with the Ru buffer sample. This trend is well explained by the bilinear and biquadratic coupling coefficients, A12 and B12, in Landau–Lifshitz–Gilbert simulations, suggesting the possibility of using both AFM and FM properties by controlling the quasi-AFM domain size.

We carried out polarized neutron reflectivity (PNR) analysis to determine the fine magnetic structure of magnetic multilayers with quasi-antiferromagnetic (quasi-AFM) layers realized by 90-deg coupling using two Co90Fe10 layers, and quantitatively evaluated the magnetization of quasi-AFM layers. Two types of samples with different buffer layers, Ru buffer and a NiFeCr buffer, were investigated and the average angles between the respective magnetization of the two Co90Fe10 layers were estimated to be +/− 39 degrees and +/− 53 degrees. In addition, less roughness was found in the NiFeCr buffer sample resulting stronger 90-deg coupling. A perfect quasi-AFM is expected to be realized by a flat interface of the magnetic multilayer.

In this study, we fabricated quasi-antiferromagnetic (AFM) layers and investigated the magnetic dynamics of quasi-AFM in both an experiment and simulation. Quasi-AFM has multi domains with alternating antiparallel magnetization, which can be realized by using 90°magnetic coupling between two ferromagnetic layers. In magnetic resonance measurement, a frequency and damping constant of CoFe-based quasi-AFM are higher than those of conventional CoFe. Likewise, in micromagnetic simulation, we obtained the spin torque oscillation in Quasi-AFM with high frequency. This suggests the possibility of a novel material with the high frequency wave generator without a stray field, like antiferromagnetic materials.

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