Abstract. Aerosols at the top of the planetary boundary layer (PBL) could modify its atmospheric dynamics by redistributing the solar radiation and start to be activated to form low-level cloud at this layer. Black carbon (BC), as an aerosol component efficiently absorbing solar radiation, can introduce heating and positive radiative effects at this sensitive layer, especially in the polluted PBL over the continent. This study presents continuous measurements of detailed BC properties at a mountain site located at the top of the polluted PBL over the North China Plain, during seasons (3 and 4 weeks of data during winter and summer, respectively) with contrasting emission structure and meteorology. The pollution level was persistently influenced by local surface anthropogenic emission on a daily basis through daytime convective mixing, but the concentration was also enhanced or diluted depending on air mass direction, defined as a neutral, polluted and diluted PBL, respectively. Winter was observed to have a higher BC mass fraction (4 %–8 %) than summer (2 %–7 %). By resolving the detailed particle size-resolved mixing state of BC in optical and hygroscopic models, we found an enhanced BC mass absorption cross section (MACBC) for the polluted PBL (up to 13 m2 g−1 at λ = 550 nm), which was 5 % higher during summer than winter due to a smaller BC core size. The higher BC mass fraction in winter corresponded to a lower single-scattering albedo by 0.03–0.09 than summer, especially the lowest for the diluted winter PBL (0.86 ± 0.02). The water supersaturation (SS) required to activate half the number of BC decreased from 0.21 % ± 0.08 % to 0.1 % ± 0.03 % for the winter diluted and polluted PBL and from 0.22 % ± 0.06 % to 0.17 % ± 0.05 % for summer. Notably, at the top of the anthropogenically polluted PBL in both seasons, the enlarged BC with enhanced absorption capacity could also be efficiently droplet activated; e.g. winter (summer) BC with an MAC of 9.84 ± 1.2 (10.7 ± 1) m2 g−1 could be half activated at SS = 0.13 % ± 0.06 % (0.18 % ± 0.05 %). This BC at the top of the PBL can more directly interact with the free troposphere and be transported to a wider region, exerting important direct and indirect radiative impacts.
A squall line is a type of strongly organized mesoscale convective system that can cause severe weather disasters. Thus, it is crucial to explore the dynamic structure and hydrometeor distributions in squall lines. This study analyzed a squall line over Guangdong Province on 6 May 2016 that was observed using a Ka-band millimeter-wave cloud radar (CR) and an S-band dual-polarization radar (PR). Doppler spectral density data obtained by the CR were used to retrieve the vertical air motions and raindrop size distribution (DSD). The results showed the following: First, the CR detected detailed vertical profiles and their evolution before and during the squall line passage. In the convection time segment (segment B), heavy rain existed with a reflectivity factor exceeding 35 dBZ and a velocity spectrum width exceeding 1.3 m s−1. In the PR detection, the differential reflectivity factor (Zdr) was 1–2 dB, and the large specific differential phase (Kdp) also represented large liquid water content. In the transition and stratiform cloud time segments (segments B and C), the rain stabilized gradually, with decreasing cloud tops, stable precipitation, and a 0 °C layer bright band. Smaller Kdp values (less than 0.9) were distributed around the 0 °C layer, which may have been caused by the melting of ice crystal particles. Second, from the CR-retrieved vertical air velocity, before squall line passage, downdrafts dominated in local convection and weak updrafts existed in higher-altitude altostratus clouds. In segment B, the updraft air velocity reached more than 8 m s−1 below the 0 °C layer. From segments C to D, the updrafts changed gradually into weak and wide-ranging downdrafts. Third, in the comparison of DSD values retrieved at 1.5 km and DSD values on the ground, the retrieved DSD line was lower than the disdrometer, the overall magnitude of the DSD retrieved was smaller, and the difference decreased from segments C to D. The standardized intercept parameter (Nw) and shape parameter (μ) of the DSD retrieved at 1.8 km showed good agreement with the disdrometer results, and the mass-weighted mean diameter (Dm) was smaller than that on the ground, but very close to the PR-retrieved Dm result at 2 km. Therefore, comparing with the DSD retrieved at around 2 km, the overall number concentration remained unchanged and Dm got larger on the ground, possibly reflecting the process of raindrop coalescence. Lastly, the average vertical profiles of several quantities in all segments showed that, first of all, the decrease of Nw and Dm with height in segments C and D was similar, reflecting the collision effect of falling raindrops. The trends were opposite in segment B, indicating that raindrops underwent intense mixing and rapid collision and growth in this segment. Then, PR-retrieved Dm profiles can verify the rationality of the CR-retrieved Dm. Finally, a vertical velocity profile peak generated a larger Dm especially in segments C and D.
Hydrometeor classification remains a challenge in winter precipitation cloud systems. To address this issue, 42 snowfall events were investigated based on a multi-platform radar observation system (i.e., X-band dual-polarization radar, Ka-band millimeter wave cloud radar, microwave radiometer, airborne equipment, etc.) in the mountainous region of northern China from 2016 to 2020. A fuzzy logic classification method is proposed to identify the particle phases, and the retrieval result was further verified with ground-based radar observation. Moreover, the hydrometeor characteristics were compared with the numerical simulations to clarify the reliability of the proposed hydrometeor classification approach. The results demonstrate that the X-/Ka- band radars are capable of identifying hydrometeor phases in winter precipitation in accordance with both ground observations and numerical simulations. Three particle categories, including snow, graupel and the mixture of snow and graupel are also detected in the winter precipitation cloud system, and there are three vertical layers identified from top to bottom, including the ice crystal layer, snow-graupel mixed layer and snowflake layer. Overall, this study has the potential for improving the understanding of microphysical processes such as freezing, deposition and aggregation of ice crystal particles in the winter precipitation cloud system.
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