We present an ultrabroadband thin-film infrared absorber made of sawtoothed anisotropic metamaterial. Absorptivity of higher than 95% at normal incidence is supported in a wide range of frequencies, where the full absorption width at half-maximum is about 86%. Such property is retained well at a very wide range of incident angles too. Light of shorter wavelengths are harvested at upper parts of the sawteeth of smaller widths, while light of longer wavelengths are trapped at lower parts of larger tooth widths. This phenomenon is explained by the slowlight modes in anisotropic metamaterial waveguide. Our study can be applied in the field of designing photovoltaic devices and thermal emitters.

A microwave ultra-broadband polarization-independent metamaterial absorber is demonstrated. It is composed of a periodic array of metal-dielectric multilayered quadrangular frustum pyramids. These pyramids possess resonant absorption modes at multi-frequencies, of which the overlapping leads to the total absorption of the incident wave over an ultra-wide spectral band. The experimental absorption at normal incidence is above 90% in the frequency range of 7.8−14.7GHz, and the absorption is kept large when the incident angle is smaller than 60 degrees. The experimental results agree well with the numerical simulation.

Electromagnetic absorbers have drawn increasing attention in many areas. A series of plasmonic and metamaterial structures can work as efficient narrowband absorbers due to the excitation of plasmonic or photonic resonances, providing a great potential for applications in designing selective thermal emitters, biosensing, etc. In other applications such as solar-energy harvesting and photonic detection, the bandwidth of light absorbers is required to be quite broad. Under such a background, a variety of mechanisms of broadband/multiband absorption have been proposed, such as mixing multiple resonances together, exciting phase resonances, slowing down light by anisotropic metamaterials, employing high loss materials and so on.

A nearly omni-directional THz absorber for both transverse electric (TE) and transverse magnetic (TM) polarizations is proposed. Through the excitation of magnetic polariton in a metal-dielectric layer, the incident light is perfectly absorbed in a thin thickness which is about 25 times smaller than the resonance wavelength. By simply stacking several such structural layers with different geometrical dimensions, the bandwidth of this strong absorption can be effectively enhanced due to the hybridization of magnetic polaritons in different layers.

Radiation absorbers have increasingly been attracting attention as crucial components for controllable thermal emission, energy harvesting, modulators, etc. However, it is still challenging to realize thin absorbers which can operate over a wide spectrum range. Here, we propose and experimentally demonstrate thin, broadband, polarization-insensitive and omnidirectional absorbers working in the near-infrared range. We choose titanium (Ti) instead of the commonly used gold (Au) to construct nano-disk arrays on the top of a silicon dioxide (SiO2) coated Au substrate, with the quality (Q) factor of the localized surface plasmon (LSP) resonance being decreased due to the intrinsic high loss of Ti. The combination of this low-Q LSP resonance and the propagating surface plasmon (PSP) excitation resonance, which occur at different wavelengths, is the fundamental origin of the broadband absorption. The measured (at normal light incidence) absorption is over 90% in the wavelength range from 900 nm to 1825 nm, with high absorption persisting up to the incident angle of ~40°. The demonstrated thin-film absorber configuration is relatively easy to fabricate and can be realized with other properly selected materials.

We experimentally demonstrate an infrared broadband absorber for TM polarized light based on an array of nanostrip antennas of several different sizes. The broadband property is due to the collective effect of magnetic responses excited by these nano-antennas at distinct wavelengths. By manipulating the differences of the nanostrip widths, the measured spectra clearly validate our design for the purpose of broadening the absorption band. The present broadband absorber works very well in a wide angular range.In the last decade, plasmonic nano-antennas have experienced a drastical boom period due to their enormous capability to compress light into a subwavelength region with an extremely strong amplitude. 1,2 To date, they have found significant application in diverse areas including sensor detection, 3 solar power harvesting, 4 thermal emission, 5 biomedical imaging, 6 ultrafast modulating, 7 etc. Patterned plasmonic antennas play a significant role for the design of thin film light absorbers, which suppress both the transmission and the reflection while maximizing the absorption. The first perfect absorber that composed by metallic split ring resonators and cutting wires was demonstrated by Landy et. al. 8 Then, it was followed by some work to improve the angular and polarization performance. [9][10][11][12] Nevertheless, all of the above absorbers work at a single band frequency which limits the pragmatic applications such as THz multi-frequency spectroscopy detection. 13 By incorporating different patterns of metallic elements, two dual band absorbers were carried out by different groups. 14,15 Recently, it was reported that based on an H-shaped nano-resonator array, a dual band plasmonic metamaterial absorber could also be constructed. 16 But they are still limited to a relative narrow band response. So far, to design a thin film absorber with broadband spectrum is still quite challenge. In our group, we have made some efforts in this aspect, by stacking multiple layers of metallic crosses with different geometrical dimensions to merge several closely positioned resonant peaks in the absorption spectrum. 17 However, this proposal suffers from one crucial drawback, namely that in the fabrication it is difficult to obtain perfect alignment to match the relative position of each pattern in different layers.It is well known that a three layered structure composed by an array of plasmonic nanostrip antennas of a fixed width on top of a ground reflecting mirror and a very thin spacer layer 18 can efficiently absorb electromagnetic wave at a certain frequency. The principle of the light absorbing is that the upper strip and the ground metal layer support a pair of anti-parallel dipoles with quite closed distance in-between, the interference of those two dipoles in far field is destructive due to their π shift phase difference so that the reflection can be totally cancelled.In this letter, also aiming at broadening the absorption band, we borrow the concept of the collective effect of multiple different oscillators 1...

Shape-morphing magnetic soft materials, composed of magnetic particles in a soft polymer matrix, can transform shape reversibly, remotely, and rapidly, finding diverse applications in actuators, soft robotics, and biomedical devices. To achieve on-demand and sophisticated shape morphing, the manufacture of structures with complex geometry and magnetization distribution is highly desired. Here, a magnetic dynamic polymer (MDP) composite composed of hard-magnetic microparticles in a dynamic polymer network with thermally responsive reversible linkages, which permits functionalities including targeted welding for magnetic-assisted assembly, magnetization reprogramming, and permanent structural reconfiguration, is reported. These functions not only provide highly desirable structural and material programmability and reprogrammability but also enable the manufacturing of functional soft architected materials such as 3D kirigami with complex magnetization distribution. The welding of magnetic-assisted modular assembly can be further combined with magnetization reprogramming and permanent reshaping capabilities for programmable and reconfigurable architectures and morphing structures. The reported MDP are anticipated to provide a new paradigm for the design and manufacture of future multifunctional assemblies and reconfigurable morphing architectures and devices.

With the potential uses of photothermal therapy (PTT) in cancer treatment with excellent efficacy, and the growing concerns about the nanotoxicity of hyperthermia agents such as carbon nanotubes and gold-based nanomaterials, the importance of searching for a biocompatible hyperthermia agent cannot be emphasized too much. In this work, a novel promising hyperthermia agent employing magnetic Fe3O4 particles with fairly low toxicity was proposed. This hyperthermia agent showed rapid heat generation under NIR irradiation. After modification with carboxymethyl chitosan (CMCTS), the obtained Fe3O4@CMCTS particles could disperse stably in PBS and serum without any aggregation. The modification of CMCTS could decrease the adsorption of bovine serum albumin (BSA) and improve the cellular uptake. In a comparative study with hollow gold nanospheres (HAuNS), Fe3O4@CMCTS particles exhibited a comparable photothermal effect and fairly low cytotoxicity. The in vivo magnetic resonance (MR) images of mice revealed that by attaching a magnet to the tumor, Fe3O4@CMCTS particles accumulated in the tumor after intravenous injection and showed a low distribution in the liver. After being exposed to a 808 nm laser for 5 min at a low power density of 1.5 W cm(-2), the tumors on Fe3O4@CMCTS-injected mice reached a temperature of ~52 °C and were completely destroyed. Thus, a kind of multifunctional magnetic nanoparticle with extremely low toxicity and a simple structure for simultaneous MR imaging, targeted drug delivery and photothermal therapy can be easily fabricated.