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High‐gain, low‐weight, wide bandwidth, and miniaturized lens antennas with stable properties against temperature are intensely required in extreme environments such as aerospace field. However, high‐performance microwave dielectric ceramics with near‐zero thermal expansion and frequency shift with temperature are very rare; moreover, the requirement of 3D printing processes also restricts their developments. Ba0.4Sr0.6Zn2Si2O7 with negative coefficient of thermal expansion (CTE), which originates from the stretched [ZnO4] tetrahedral chain to the twisted one along b‐axis with temperature, and CaTiO3 with positive temperature coefficient of resonant frequency (τf) can effectively adjust both CTE and τf of Zn1.8SiO3.8 to near‐zero value in 0.95(0.9Zn1.8SiO3.8–0.1Ba0.4Sr0.6Zn2Si2O7)–0.05CaTiO3 ceramic. Then, a Ku‐band Luneburg lens integrative antenna fabricated by stereolithography 3D printing technology exhibits an average gain of 8.06 dBi at 10.45–11.39 GHz and 10.3 dBi at 12.27–13.45 GHz, which has potential applications in temperature‐stable satellite communication.

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