Although Ti 3 C 2 T x MXene/fabric composites have shown promise as flexible pressure sensors, the effects of MXene composition and structure on piezoresistive properties and the effects of the textile structure on sensitivity have not been systematically studied. Herein, impregnation at room temperature was used as a cost-effective and scalable method to prepare composite materials using different fabrics [plain-woven fabric, twill-woven fabric, weft plain-knitted fabric, jersey cross-tuck fabric, and nonwoven fabric (NWF)] and MXene nanosheets (Ti 3 C 2 T x , Ti 2 CT x , Ti 3 CNT x , Mo 2 CT x , Nb 2 CT x , and Mo 2 TiC 2 T x ). The MXene nanosheets adhered to the fabric surface through hydrogen bonding, resulting in a conductive network structure. The Ti 3 C 2 T x @NWF composite was found to be the optimal flexible pressure sensor, demonstrating high sensitivity (6.31 kPa −1 ), a wide sensing range (up to 150 kPa), fast response/recovery times (300 ms/260 ms), and excellent durability (2000 cycles). Furthermore, the sensor was successfully used to monitor full-scale human motion, including pulse, and a 4 × 4 pixel flexible sensor array was shown to accurately locate pressure and recognize the pressure magnitude. These findings provide a basis for the rational design of MXene/textile composites as wearable pressure sensors for medical diagnosis, human−computer interactions, and electronic skin applications.

Soft robots are those that can move like living organisms and adapt to the surrounding environment. Compared with traditional rigid robots, the advantages of soft robots, in terms of material flexibility, human–computer interaction, and biological adaptability, have received extensive attention. Flexible actuators based on light response are one of the most promising ways to promote the field of cordless soft robots, and they have attracted the attention of scientists in bionic design, actuation implementation, and application. First, the three working principles and the commonly used light-responsive materials for light-responsive actuators are introduced. Then, the characteristics of light-responsive soft actuators are sequentially presented, emphasizing the structure strategy, actuation performance, and emerging applications. Finally, this review is concluded with a perspective on the existing challenges and future opportunities in this nascent research frontier.

Highly conductive, flexible, stretchable and lightweight electrode substrates are essential to meet the future demand on supercapacitors for wearable electronics. However, it is difficult to achieve the above characteristics simultaneously. In this study, ultrafine stainless-steel fibers (with a diameter of ≈30 μm) are knitted into stainless-steel meshes (SSMs) with a diamond structure for the fabrication of textile stretchable electrodes and current collectors. The electrodes are fabricated by utilizing an electrodeposited three-dimensional network graphene framework and poly(3,4-ethylenedioxythiophene) (PEDOT) coating on the SSM substrates via a two-step electrodeposition process, which show a specific capacitance of 77.09 F g−1 (0.14 A g−1) and superb cycling stability (91% capacitance retention after 5000 cycles). Furthermore, the assembled flexible stretchable supercapacitor based on the PEDOT/reduced graphene oxide (RGO)@SSM electrodes exhibits an areal capacitance (53 mF cm−2 at 0.1 mA cm−2), a good cycling stability (≈73% capacitance retention after 5000 cycles), rate capability (36 mF cm−2 at 5 mA cm−2), stretchable stability (≈78% capacitance retention at 10% strain for 500 stretching cycles) and outstanding flexibility and stability under various bending deformations. The assembled supercapacitors can illuminate a thermometer and a light-emitting diode, demonstrating their potential application as stretchable supercapacitors. This simple and low-cost method developed for fabricating lightweight, stretchable and stable high-performance supercapacitors offers new opportunities for future stretchable electronic devices.

Flexible wearable strain sensors with excellent sensing performance have received widespread interest due to their superior application capability in the field of human-computer interaction, sports rehabilitation, and disease diagnosis. But at present, it is still a considerable challenge to exploit a flexible strain sensor with high sensitivity and wide sensing range that is easily manufactured, low-cost, and easily integrable into clothing. MXene is a promising material sensitive enough for flexible sensors due to its superior conductivity and hydrophilicity. The warp knitting weft insertion textile structure gives the fabric excellent elasticity, making it suitable as a flexible, stretchable substrate. Therefore, utilizing a polyester elastic fabric with a warp knitting weft insertion structure, a fabric strain sensor with high sensitivity and wide sensing range prepared by layer-by-layer self-assembly of polyvinyl alcohol layers and MXene layers is reported in this study. The strain sensor exhibits high sensitivity (up to 288.43), a wide sensing range (up to 50%), fast response time (50 ms), ultra-low detection limit (a strain of 0.067%), excellent cycle stability (1000 cycles), and good washability. Besides, affixing the MXene/polyvinyl alcohol/polyester elastic fabric strain sensor on the joints can detect the movement of limbs. Therefore, the MXene/polyvinyl alcohol/polyester elastic fabric strain sensor demonstrates potential application opportunities in smart wearable electronic devices, and the researcher can also apply this method in the production of other flexible, intelligent wearable devices.

No abstract