The OHC shows superior performance as an anode material for LIBs with a high reversible capacity (1181 mA h g−1 at 0.1 A g−1) and an excellent rate capability (304 mA h g−1 at 5 A g−1).
A facile, economical and effective method to produce hierarchically porous nitrogen-rich carbon (HPNC) from wheat straw has been reported. Acid pretreatment is introduced before KOH activation, and plays the role of promoting the formation of thinner pore walls. Without any N-doping, the N content is as high as 5.13%. The HPNC when used as an anode for Li-ion batteries exhibits a superior specific capacity of 1470 mA h g À1 at 0.037 A g À1 , and possesses an ultrahigh rate capability of 344 mA h g À1 at 18.5 A g À1 . Even at an extremely high current density of 37 A g À1 , the reversible capacity is still as high as 198 mA h g À1 .
A flexible heterostructure is reported herein, which elastically couples the volumetric variation during SCO to the electrical conductivity of a strain-sensitive metallic conductor, thereby resulting in synergistic electrical bistability.
The recently discovered 12442-type ACa2Fe4As4F2 (A = K, Rb, Cs) compounds are the only iron-based superconductors (IBSs) with double FeAs layers between neighboring insulating layers, analogous to the double CuO2 layers in some high-T
c cuprates. Here, we report the study of vortex phase diagram of RbCa2Fe4As4F2 single crystal via magneto-transport and magnetization measurements. The resistive transition under magnetic fields shows a foot-like kink at a characteristic temperature, T
s, followed by a resistive tail in nearly zero resistivity region. Such behavior is ascribed to a vortex slush transition at T
s, below which the vortex state has short-range vortex lattice correlation, and then a second-order transition into the vortex glass phase occurs with further decreasing temperature. Above T
s, the Arrhenius plot of resistivity shows two linear regions that are separated by a crossover line T
cr(B), which is associated with a crossover from collective to plastic pinning or different flux pinning behaviors resulted from different types of defect. In addition, the magnetic hysteresis loops reveal a second magnetization peak (SMP), which is shifted to lower fields with increasing temperature for T< 12 K. However, the SMP unexpectedly moves back to a higher field at T= 12 K, and then gradually turns into a shoulder or kink that moves to higher fields at high temperatures, such anomalous behavior has never been observed in IBSs. According to the magneto-transport and magnetization data, the vortex phase diagram of RbCa2Fe4As4F2 is finally constructed. Details on the different vortex phase transitions and relevant physical scenarios are given and discussed.
Two new two-stage manipulation protocols, namely light- and temperature-assisted spin state annealing (LASSA/TASSA), are applied to a spin crossover coordination polymer, [Fe(isoq)2{Au(CN)2}2], revealing the hidden multistability of spin states.
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