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Magnetic and transport properties of near stoichiometric metastable FexMnyGaz alloys (46 ≤ x ≤ 52, 17 ≤ y ≤ 25, 26 ≤ z ≤ 30) with face-centered cubic (FCC), body-centered cubic (BCC), and two-phase (FCC + BCC) structures are investigated. The experimental results are analyzed in terms of first-principles calculations of stoichiometric Fe2MnGa alloy with the L21, L12, and the tetragonally distorted L21 structural orderings. It is shown that the pure BCC and FCC phases have distinct magnetic and transport properties. Two-phase Fe2MnGa alloys have magnetic and transport properties typical of the mixed BCC and FCC phases. Among the investigated alloys, Fe46Mn24Ga30 has a martensitic transformation accompanied with significant changes of its magnetic and transport properties.

The structural dependence of the magnetic, transport, optical, and magneto-optical (MO) properties of Cu2MnAl Heusler alloy (HA) thin-film samples was investigated. Disordered thin films of Cu2MnAl HA fabricated by vapor-quenching deposition onto substrates cooled by liquid nitrogen behave as highly resistive Pauli paramagnets down to 5 K, while an annealing of the disordered films at 580 K for 1 h restores the L21-type ordered structure, as well as the ferromagnetic order and other physical properties typical for the ordered Cu2MnAl HA film. The film deposition onto substrates held at T⩾690K leads to the formation of a multiphase crystalline structure. A significant influence of the structural disorder on the optical and MO properties of Cu2MnAl was experimentally observed and discussed in terms of the electronic structure of the alloy.