An electron hopping on non-coplanar spin sites with spin chirality obtains a complex phase factor (Berry phase) in its quantum mechanical amplitude that acts as an internal magnetic field, and is predicted to manifest itself in the Hall effect when it is not cancelled. The present combined work of transport measurement, neutron scattering, and theoretical calculation provides evidence that the gigantic anomalous Hall effect observed in Nd2Mo2O7, a pyrochlore ferromagnet with geometrically frustrated lattice structure, is mostly due to the spin chirality and the associated Berry phase originating from the Mo spin tilting.

Geometrically frustrated magnets provide abundant opportunities for discovering complex spin textures, which sometimes yield unconventional electromagnetic responses in correlated electron systems. It is theoretically predicted that magnetic frustration may also promote a topologically nontrivial spin state, i.e., magnetic skyrmions, which are nanometric spin vortices. Empirically, however, skyrmions are essentially concomitant with noncentrosymmetric lattice structures or interfacialsymmetry-breaking heterostructures. Here, we report the emergence of a Bloch-type skyrmion state in the frustrated centrosymmetric triangular-lattice magnet Gd2PdSi3. We identified the field-induced skyrmion phase via a giant topological Hall response, which is further corroborated by the observation of in-plane spin modulation probed by resonant x-ray scattering. Our results exemplify a new gold mine of magnetic frustration for producing topological spin textures endowed with emergent electrodynamics in centrosymmetric magnets.

Skyrmions, topologically protected vortex-like nanometric spin textures in magnets, have been attracting increasing attention for emergent electromagnetic responses and possible technological applications for spintronics. In particular, metallic magnets with chiral and cubic/tetragonal crystal structure may have high potential to host skyrmions that can be driven by low electrical current excitation. However, experimental observations of skyrmions have been limited to below room temperature for the metallic chiral magnets, specifically for the MnSi-type B20 compounds. Towards technological applications, transcending this limitation is crucial. Here we demonstrate the formation of skyrmions with unique spin helicity both at and above room temperature in a family of cubic chiral magnets: β-Mn-type Co-Zn-Mn alloys with a different chiral space group from that of B20 compounds. Lorentz transmission electron microscopy, magnetization and small-angle neutron scattering measurements unambiguously reveal formation of a skyrmion crystal under application of a magnetic field in both thin-plate and bulk forms.

Controlling ferromagnetism by an external electric field has been a great challenge in materials physics, for example towards the development of low-power-consumption spintronics devices. To achieve an efficient mutual control of electricity and magnetism, the use of multiferroics--materials that show both ferroelectric and ferromagnetic/antiferromagnetic order--is one of the most promising approaches. Here, we show that GdFeO(3), one of the most orthodox perovskite oxides, is not only a weak ferromagnet but also possesses a ferroelectric ground state, in which the ferroelectric polarization is generated by the striction through the exchange interaction between the Gd and Fe spins. Furthermore, in this compound, ferroelectric polarization and magnetization are successfully controlled by magnetic and electric fields, respectively. This unprecedented mutual controllability of electricity and magnetism is attributed to the unique feature of composite domain wall clamping of the respective domain walls for electric and magnetic orders. This domain wall feature generally determines the efficiency of the mutual controllability and thus could have an important role towards the application of multiferroics to practical devices.

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We present an angle-resolved photoemission doping dependence study of the n-type cuprate superconductor Nd(2-x)Ce(x)CuO(4+/-delta), from the half-filled Mott insulator to the T(c) = 24 K superconductor. In Nd2CuO4, we reveal the charge-transfer band for the first time. As electrons are doped into the system, this feature's intensity decreases with the concomitant formation of near- E(F) spectral weight. At low doping, the Fermi surface is an electron-pocket (with volume approximately x) centered at (pi,0). Further doping leads to the creation of a new holelike Fermi surface (volume approximately 1+x) centered at (pi,pi). These findings shed light on the Mott gap, its doping evolution, as well as the anomalous transport properties of the n-type cuprates.

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PACS numbers:2 Skyrmions, topologically-protected nanometric spin vortices, are being investigated 1-11 extensively in various magnets.Among them, many of structurally-chiral cubic magnets host the triangular-lattice skyrmion crystal (SkX) as the thermodynamic equilibrium state. However, this state exists only in a narrow temperature and magnetic-field region just below the magnetic transition temperature T c , while a helical or conical magnetic state prevails at lower temperatures. Here we describe that for a room-temperature skyrmion material 12 , β-Mn-type Co 8 Zn 8 Mn 4 , a field-cooling via the equilibrium SkX state can suppress the transition to the helical or conical state, instead realizing robust metastable SkX states that survive over a very wide temperature and magnetic-field region, including down to zero temperature and up to the critical magnetic field of the ferromagnetic transition. Furthermore, the lattice form of the metastable SkX is found to undergo reversible transitions between a conventional triangular lattice and a novel square lattice upon varying the temperature and magnetic field. These findings exemplify the topological robustness of the once-created skyrmions, and establish metastable skyrmion phases as a fertile ground for technological applications. Skyrmions are promising for spintronics applications firstly because they are stable due to their topological nature, and secondly because they can be manipulated by an ultra-low current density [17][18][19][20][21] . The recent discovery of skyrmion formation at and above room temperature in a new group of chiral magnets, β-Mn-type Co-Zn-Mn alloys, has provided a significant step toward applications 12 . These materials possess a chiral cubic crystal structure with space group P 4 1 32 as shown in Fig. 1 A square-lattice SkX state, characterized by double-q vectors orthogonal to each other and perpendicular to the magnetic field, also shows up as a 4 spot pattern in the H beam geometry. In the H ⊥ beam geometry, the helical multi-domain state shows 4 spots, the conical state 2 spots on the horizontal axis, and both the triangular and square-lattice SkX states each 2 spots on the vertical axis.Keeping the above relations in mind, we next consider the results (Fig. 3) of the FC process at 0.04 T, i.e. by way of the thermodynamical equilibrium triangular-lattice SkX region (green region in Fig. 1(b)). The SANS images in Fig. 3(b) show that the pattern obtained from the equilibrium triangular-lattice SkX generated at 295 K persists down to 200K. This is a direct demonstration of the realization of the metastable SkX state that exists outside of the equilibrium state for temperatures below 284 K. The lifetime of this metastable SkX is very long and becomes essentially time-independent below 260 K ( Supplementary Fig. S4). At 120 K, the triangular-lattice SkX pattern has partially transformed into 4 spots.At 40 K, the 4 spots become clearer and their |q|(≡ q) values become larger than they were 6 at higher temperatures. The 4 spot patter...