In recent years, graphene has emerged as potential reinforcing nanofiller in the composites for structural engineering due to its extraordinary high elastic modulus and mechanical strength. As recognized, the transfer of stress from a low modulus matrix to a high-modulus reinforcing graphene and the interfacial behavior at a graphene-matrix interface is the fundamental issue in these composites. In the case of graphene nanosheet (GNS) reinforced hydroxyapatite (HA) composite, this research presented analytical models and simulated that the number of graphene layers of GNSs has little effect on the maximum axial stress (∼0.35 GPa) and the maximum shear stress (∼0.14 GPa) at a GNS-HA interface, and the energy dissipation by GNS pull-out decreases with increasing the number of graphene layers due to weak bonding between them. Also, GNS-HA interfacial delamination and/or GNS rupture were also indentified to be the two key failure mechanisms. The computed results are expected to facilitate a better understanding of the interfacial behavior at a GNS-ceramic interface and to achieve tough ceramics reinforced with GNSs.
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