A novel model named random-forest-spatiotemporal-kriging (RF-STK) was developed to estimate the daily ambient NO concentrations across China during 2013-2016 based on the satellite retrievals and geographic covariates. The RF-STK model showed good prediction performance, with cross-validation R = 0.62 (RMSE = 13.3 μg/m) for daily and R = 0.73 (RMSE = 6.5 μg/m) for spatial predictions. The nationwide population-weighted multiyear average of NO was predicted to be 30.9 ± 11.7 μg/m (mean ± standard deviation), with a slowly but significantly decreasing trend at a rate of -0.88 ± 0.38 μg/m/year. Among the main economic zones of China, the Pearl River Delta showed the fastest decreasing rate of -1.37 μg/m/year, while the Beijing-Tianjin Metro did not show a temporal trend ( P = 0.32). The population-weighted NO was predicted to be the highest in North China (40.3 ± 10.3 μg/m) and lowest in Southwest China (24.9 ± 9.4 μg/m). Approximately 25% of the population lived in nonattainment areas with annual-average NO > 40 μg/m. A piecewise linear function with an abrupt point around 100 people/km characterized the relationship between the population density and the NO, indicating a threshold of aggravated NO pollution due to urbanization. Leveraging the ground-level NO observations, this study fills the gap of statistically modeling nationwide NO in China, and provides essential data for epidemiological research and air quality management.

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