The emergence of a topologically nontrivial vortex-like magnetic structure, the magnetic skyrmion, has launched new concepts for memory devices. Extensive studies have theoretically demonstrated the ability to encode information bits by using a chain of skyrmions in one-dimensional nanostripes. Here, we report experimental observation of the skyrmion chain in FeGe nanostripes by using high-resolution Lorentz transmission electron microscopy. Under an applied magnetic field, we observe that the helical ground states with distorted edge spins evolve into individual skyrmions, which assemble in the form of a chain at low field and move collectively into the interior of the nanostripes at elevated fields. Such a skyrmion chain survives even when the width of the nanostripe is much larger than the size of single skyrmion. This discovery demonstrates a way of skyrmion formation through the edge effect, and might, in the long term, shed light on potential applications.

Magnetic skyrmion is a nanosized magnetic whirl with nontrivial topology, which is highly relevant for applications on future memory devices. To enable the applications, theoretical efforts have been made to understand the dynamics of individual skyrmions in magnetic nanostructures. However, directly imaging the evolution of highly geometrically confined individual skyrmions is challenging. Here, we report the magnetic field-driven dynamics of individual skyrmions in FeGe nanodisks with diameters on the order of several skyrmion sizes by using Lorentz transmission electron microscopy. In contrast to the conventional skyrmion lattice in bulk, a series of skyrmion cluster states with different geometrical configurations and the fielddriven cascading phase transitions are identified at temperatures far below the magnetic transition temperature. Furthermore, a dynamics, namely the intermittent jumps between the neighboring skyrmion cluster states, is found at elevated temperatures, at which the thermal energy competes with the energy barrier between the skyrmion cluster states.T he complex spin configurations in helimagnets have attracted considerable attention recently, with the topologically stable particle-like spin texture with a size down to the nanoscale, namely magnetic skyrmion, as the focus of interest (1). Magnetic skyrmion is characterized as a nanoscale topological particle producing unconventional spin electronic phenomena (2, 3) that holds great promise for future spintronic devices, including racetrack memory (4), magnetic random access memory, and magnetic sensors (1). Essentially, such schemes rely on the controllable formation and manipulation of individual skyrmions at nanostructured elements with various shapes such as disks, stripes, or wires (5-7). Investigation of skyrmions in confined geometries has therefore become one of the major topics in the field of skyrmion physics (5-10).Unlike ordinary magnetic vortices in microsized soft magnetic disks due to the minimization of the dipolar energy (11), the key ingredient of stabilizing skyrmions in helimagnets is the antisymmetry Dzyaloshinskii−Moriya (DM) interactions originating from the broken inversion symmetry (12). The competition of the DM coupling with ferromagnetic exchange interaction results in periodic helical ground state in helimagnets. Under the action of a magnetic field and temperature, these magnetic helices transfer into skyrmion crystal with triangular lattice configuration, and finally to the field-polarized ferromagnetic state. Notably, both ferromagnetic and DM couplings occur among the neighboring spins and belong to short-range interaction. Thus, it was demonstrated theoretically that skyrmions cluster states, characterized by certain arrangements of limited skyrmions, still persist even in submicrometer objects (8, 13). There, the longrange lattice form of skyrmions in 2D or bulk helimagnets is broken, but a short-ranged ordering with specific geometrical symmetries still remains, and the number of skyrmions in the cluster...

A tunable response frequency is highly desirable for practical applications of microwave absorption materials but remains a great challenge. Here, hollow lightweight polydopamine@α-MnO2 microspindles were facilely synthesized with the tunable absorption frequency governed by the aspect ratio. The size of the hard template is a key factor to achieve the unique shape; the polymer layer with uniform thickness plays an important role in obtaining spindles with homogeneous size. With the aspect ratio increasing, the maximum reflection loss, as well as the absorption bandwidth (<-10 dB), increases and then decreases; meanwhile, the microwave absorption band shifts to the low frequency. The optimized aspect ratio of the cavity about the hollow polydopamine@α-MnO2 microspindles is ∼2.8. With 3 mm thickness at 9.7 GHz, the strongest reflection reaches -21.8 dB, and the width of the absorbing band (<-10 dB) is as wide as 3.3 GHz. Via electron holography, it is confirmed that strong charge accumulates around the interface between the polydopamine and α-MnO2 layers, which mainly contributes to the dielectric polarization absorption. This study proposes a reliable strategy to tune the absorption frequency via different aspect ratio polymer@α-MnO2 microspindles.

In this study, CoNi flower-like hierarchical microstructures with different sizes were obtained via a one-step solvothermal method by simply adjusting the concentration of precursors and surfactant. The obtained CoNi microflowers possess uniform and tunable size, good monodispersity, and remarkable magnetic microwave absorption properties as well as electron holography phase images. Characterization results have demonstrated the dependency of properties of CoNi microflowers on their morphologies and sizes. The microflowers exhibit different stray magnetic fields that might be determined by whether the pristine nanoflakes on the flowers' surface was parallel or perpendicular to grid plane. And as the size of microflowers increased, the coercive force (Hc) value decreased while saturation magnetization (Ms) value gradually increased, and it can be also observed that the values of Ms and Hc at 5 K are higher than those at 300 K. In addition, the blocking temperature decreased when size increased. Typically, the 2.5 μm CoNi microflowers achieve the maximum reflection loss (RL) value of -28.5 dB at 6.8 GHz with a thickness of 2 mm, while on the other hand, the 0.6 μm flowers achieved a broader absorption bandwidth below -10 dB of 6.5 GHz. Therefore, it is believable that the CoNi flowers with different sizes and hierarchical structures in this work have great potential for high performance magnetic microwave absorption applications.

We report direct evidence of the field-dependent character of the interaction between individual magnetic skyrmions as well as between skyrmions and edges in B20-type FeGe nanostripes observed by means of high-resolution Lorentz transmission electron microscopy. It is shown that above certain critical values of an external magnetic field the character of such long-range skyrmion interactions changes from attraction to repulsion. Experimentally measured equilibrium inter-skyrmion and skyrmion-edge distances as a function of the applied magnetic field shows quantitative agreement with the results of micromagnetic simulations. The important role of demagnetizing fields and the internal symmetry of three-dimensional magnetic skyrmions are discussed in detail.

The magnetic skyrmion is a topologically stable vortex-like spin texture that offers great promise as information carriers for future spintronic devices. In a two-dimensional chiral magnet, it was generally considered that a tilted magnetic field is harmful to its formation and stability. Here we investigated the angular-dependent stability of magnetic skyrmions in FeGe nanosheets by using high-resolution Lorentz transmission electron microscopy (Lorentz TEM). Besides the theoretically predicted destruction of skyrmion lattice state by an oblique magnetic field as the temperature closes to its magnetic Curie temperature T ∼ 278 K, we also observed an unexpected reentry-like phenomenon at the moderate temperatures near the border between conical and skyrmion phase, T ∼ 240 K. This behavior is completely beyond the theoretical prediction in a conventional two-dimensional (2D) system. Instead, a three-dimensional (3D) model involving the competition between conical phase and skyrmions is likely to play a crucial role.

Local heterogeneity in crystal lattice is directly observed in synthesized Li2MnO3/LiMO2 (M = Ni, Mn) cathode materials. With SAED application, for the first time, we accordingly uncover that the lattice heterogeneity is induced by different Li2MnO3 atomic arrangements coexisting in same crystal domain.

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