This paper demonstrates the role of meteorology and air transport in influencing the South African atmospheric CO2 distribution. CO2 data from December 2004 to December 2009 acquired by the Tropospheric Emission Spectrometer (TES) instrument onboard the Aura satellite were used to establish the CO2 vertical distribution at selected regions in South Africa. The Hybrid Single-Particle Lagrangian Integrated Trajectories (HYSPLIT) atmospheric model backward trajectories were used to determine the long-range air transport impacting on South African CO2 atmospheric distribution and to detect the source areas of air masses impacting on South Africa’s atmosphere. The study found that long-range air transport can result in the accumulation or dilution of atmospheric CO2 at various sites in South Africa, depending on the source region and type of air flow. The long-range air transport from different source regions at the upper air level between the 700 and 500 hPa stable layers and the layer above 500 hPa strengthens the inhomogeneity in the vertical distribution of CO2, which is caused by the decoupling effect of the upper air stable layers. This long-range air transport also involves intercontinental air transport.
There are two methods of harvesting sugarcane—manual or mechanical. Manual harvesting requires the burning of the standing sugarcane crop. Burning of the crop results in the emission of aerosols and harmful trace gases into the atmosphere. This work makes use of a long-term dataset (1980–2019) to study (1) the atmospheric spatial and vertical distribution of pollutants; (2) the spatial distribution and temporal change of biomass emissions; and (3) the impact/influence of climatic factors on temporal change in atmospheric pollutant loading and biomass emissions over the Mpumalanga and KwaZulu Natal provinces in South Africa, where sugarcane farming is rife. Black carbon (BC) and sulfur dioxide (SO2) are two dominant pollutants in the JJA and SON seasons due to sugarcane burning. Overall, there was an increasing trend in the emissions of BC, SO2, and carbon dioxide (CO2) from 1980 to 2019. Climatic conditions, such as warm temperature, high wind speed, dry conditions in the JJA, and SON season, favor the intensity and spread of the fire, which is controlled. The emitted pollutants are transported to neighboring countries and can travel over the Atlantic Ocean, as far as ~6600 km from the source site.
A peak in the ambient ozone concentration was observed at three of the six ambient air quality monitoring stations in the Vaal Triangle Airshed Priority Area on the second of June 2013. The ozone peak was associated with elevated concentrations of particulate matter, including PM10, PM2.5 and black carbon, but not sulphur dioxide, oxides of nitrogen, carbon monoxide nor benzene. Back trajectory analysis using Hysplit showed that the air masses containing the high levels of ozone passed over areas influenced by coal fired power stations in the Waterberg, metal processing in the Bojanala region and high intensity fires 30km to 50km upwind of the stations.
South Africa is the dominant continental source region of CO 2 fossil fuel emissions. This is a result of the strong dependence of its economy on fossil fuels. However, the observations of atmospheric CO 2 in South Africa are inadequate. The country has the Global Atmospheric Watch (GAW) Cape Point station as the only site with long-term ambient CO 2 monitoring record. In this study, satellite data retrieved from the Tropospheric Emission Spectrometer (TES) instrument on board the Aura satellite from Dec 2004 to Dec 2009 is used for the first time to quantify the spatial distribution of CO 2 over South Africa, as well as to determine its annual variability at selected sites. The study found that the surface CO 2 foot print in South Africa resembles the industrial CO 2 emission sources spatial distribution, particularly during the summer and autumn. In winter and spring seasons the surface CO 2 foot prints are spatially expanded as a result of contributions of emissions from biomass and domestic fossil fuel combustion. The surface levels of CO 2 at the study areas have been increasing during the period of the analysis.
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