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A novel mesoporous γ-Fe2O3-modified nanoflower-MnO2/attapulgite catalyst has been fabricated through a facile hydrothermal method and used for low temperature SCR of NOx with NH3.

A series of γ-MnO2-Ce/MMT catalyst materials synthesized by homogeneous precipitation method was investigated for the selective catalytic reduction (SCR) of NOx with NH3. X-ray diffraction and specific surface areas were utilized for micro structure and layer spacing investigation. And NH3-TPD, Pyridoxine IR, H2-TPR and XPS were used to investigate Brønsted acid and Lewis acid, redox properties, atomic concentrations and element chemical state for as-prepared catalysts. The results showed that the γ-MnO2-Ce/MMT had superior NOx conversion compared to the bulk particles, among which 6 wt.% γ-MnO2-Ce/MMT displayed the best deNOx of 95.3% for the low temperature selective catalytic reduction of NOx with NH3 (NH3-SCR) under the GHSV of 25,000 h−1, therefore it is a promising catalyst for low temperature NH3-SCR.

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