Aerosol‐meteorology interactions can change surface aerosol concentrations via different mechanisms such as altering radiation budget or cloud microphysics. However, few studies investigated the impacts of different mechanisms on temporal and spatial distribution of PM2.5 concentrations over China. Here we used the fully coupled Weather Research and Forecasting model with online chemistry (WRF‐Chem) to quantify the enhancement of PM2.5 concentrations by aerosol‐meteorology feedback in China in 2014 for different seasons and separate the relative impacts of aerosol radiation interactions (ARIs) and aerosol‐cloud interactions (ACIs). We found that ARIs and ACIs could increase population‐weighted annual mean PM2.5 concentration over China by 4.0 μg/m3 and 1.6 μg/m3, respectively. We found that ARIs play a dominant role in aerosol‐meteorology interactions in winter, while the enhancement of PM2.5 concentration by ARIs and ACIs is comparable in other three seasons. ARIs reduced the wintertime monthly mean wind speed and planetary boundary layer (PBL) height by up to 0.1 m/s and 160 m, respectively, but increased the relative humidity by up to 4%, leading to accumulation of pollutants within PBL. Also, ARIs reduced dry deposition velocity of aerosols by up to 20%, resulting in an increase in PM2.5 lifetime and concentrations. ARIs can increase wintertime monthly mean surface PM2.5 concentration by a maximum of 30 μg/m3 in Sichuan Basin. ACIs can also increase PM2.5 concentration with more significant impacts in wet seasons via reduced wet scavenging and enhanced in‐cloud chemistry. Dominant processes in PM2.5 enhancement are also clarified in different seasons. Results show that physical process is more important than chemical processes in winter in ARIs, while chemical process of secondary inorganic aerosols production may be crucial in wet seasons via ACIs.
In order to research the mechanical mechanism of plants anti-erosion and provide some basis to screen windbreak and soil-reinforcement specie for wind and water complex erosion area. This research selected Caragana microphylla Lam, Salix psammophila C.wang et Ch.Y.Yang, Artemisia sphaerocephala Krasch and Hippophae rhamnides Linn four kinds of soil and water conservation plants of Inner Mongolia Ordos as the research object. During the period of spring gale, thirteen indicators (single shrub reduce wind velocity ration, shelterbelt reduce wind velocity ration, community reduce wind velocity ration, taproots tensile strength, represented root constitutive properties, represented root elasticity modulus, lateral roots branch tensile strength, accumulation surface area, root-soil interface sheer strength, interface friction coefficient, length of accumulative root, root-soil composite cohesive, root-soil composite equivalent friction angle) of foliage windbreak and root mechanical properties were evaluated by the analytic hierarchy process (AHP). The results showed the index of windbreak and soil-reinforcement were in the sequence of Salix psammophila C.wang et Ch.Y.Yang (0.84) > Caragana microphylla Lam (0.45) > Artemisia sphaerocephala Krasch (-0.47) > Hippophae rhamnides Linn (-0.83). Therefore, Salix psammophila C.wang et Ch.Y.Yang could be regarded as the important anti-erosion specie for wind erosion area.
Aerosols can interact with other meteorological variables in the air via aerosol–radiation or aerosol–cloud interactions (ARIs/ACIs), thus affecting the concentrations of particle pollutants and ozone. The online-coupled model WRF-Chem was applied to simulate the changes in the PM2.5 (particulate matter less than 2.5 μm in aerodynamic diameter) and ozone concentrations that are caused by these mechanisms in China by conducting three parallel sensitivity tests. In each case, availabilities of aerosol–radiation interactions and aerosol–cloud interactions were set differently in order to distinguish each pathway. Partial correlation coefficients were also analyzed using statistical tools. As suggested by the results, the ARIs reduced ground air temperature, wind speed, and planetary boundary height while increasing relative humidity in most places. Consequently, the ozone concentration in the corresponding region declined by 4%, with a rise in the local annual mean PM2.5 concentration by approximately 12 μm/m3. The positive feedback of the PM2.5 concentration via ACIs was also found in some city clusters across China, despite the overall enhancement value via ACIs being merely around a quarter to half that via ARIs. The change in ozone concentration via ACIs exhibited different trends. The ozone concentration level increased via ACIs, which can be attributed to the drier air in the south and the diminished solar radiation that is received in central and northern China. The correlation coefficient suggests that the suppression in the planetary boundary layer is the most significant factor for the increase in PM2.5 followed by the rise in moisture required for hygroscopic growth. Ozone showed a significant correlation with NO2, while oxidation rates and radiation variance were also shown to be vitally important.
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