We present the results of birch pollen characterization using lidar and in situ measurements based on a 11 d pollination period from 5 to 15 May 2016 at the European Aerosol Research Lidar Network (EARLINET) station in Vehmasmäki (Kuopio; 62 • 44 N, 27 • 33 E), Finland. The ground-based multiwavelength Raman polarization lidar Polly XT performed continuous measurements at this rural forest site and has been combined with a Hirst-type volumetric air sampler, which measured the pollen type and concentration at roof level (4 m). The period was separated into two parts due to different atmospheric conditions and detected pollen types. During the first period, high concentrations of birch pollen were measured with a maximum 2 h average pollen concentration of 3700 grains m −3 . Other pollen types represented less than 3 % of the total pollen count. In observed pollen layers, the mean particle depolarization ratio at 532 nm was 10 ± 6 % during the intense birch pollination period. Mean lidar ratios were found to be 45±7 and 55±16 sr at 355 and 532 nm, respectively. During the second period, birch pollen was still dominant, but a significant contribution of spruce pollen was observed as well. Spruce pollen grains are highly nonspherical, leading to a larger mean depolarization ratio of 26 ± 7 % for the birch-spruce pollen mixture. Furthermore, higher lidar ratios were observed during this period with mean values of 60 ± 3 and 62 ± 10 sr at 355 and 532 nm, respectively. The presented study shows the potential of the particle depolarization ratio to track pollen grains in the atmosphere.Published by Copernicus Publications on behalf of the European Geosciences Union.
Abstract. In June 2013, a ground-based mobile lidar performed the ∼ 10 000 km ride from Paris to Ulan-Ude, near Lake Baikal, profiling for the first time aerosol optical properties all the way from western Europe to central Siberia. The instrument was equipped with N 2 -Raman and depolarization channels that enabled an optical speciation of aerosols in the low and middle troposphere. The extinction-to-backscatter ratio (also called lidar ratio or LR) and particle depolarization ratio (PDR) at 355 nm have been retrieved. The LR in the lower boundary layer (300-700 m) was found to be 63 ± 17 sr on average during the campaign with a distribution slightly skewed toward higher values that peaks between 50 and 55 sr. Although the difference is small, PDR values observed in Russian cities (> 2 %, except after rain) are systematically higher than the ones measured in Europe (< 1 %), which is probably an effect of the lifting of terrigenous aerosols by traffic on roads. Biomass burning layers from grassland or/and forest fires in southern Russia exhibit LR values ranging from 65 to 107 sr and from 3 to 4 % for the PDR. During the route, desert dust aerosols originating from the Caspian and Aral seas regions were characterized for the first time, with a LR (PDR) of 43 ± 14 sr (23 ± 2 %) for pure dust. The lidar observations also showed that this dust event extended over 2300 km and lasted for ∼ 6 days. Measurements from the Moderate Resolution Imaging Spectrometer (MODIS) show that our results are comparable in terms of aerosol optical thickness (between 0.05 and 0.40 at 355 nm) with the mean aerosol load encountered throughout our route.
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