For the performance improvement of microbial fuel cells (MFCs), the anode becomes a breakthrough point due to its influence on bacterial attachment and extracellular electron transfer (EET). On other level, carbon materials possess the following features: low cost, rich natural abundance, good thermal and chemical stability, as well as tunable surface properties and spatial structure.This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
The construction of an optimized electrolyte system compatible with layered transition metal (TM) oxides is of great importance to advanced sodium‐ion batteries (SIBs). Herein, a low‐cost iron‐containing manganese‐based layered cathode material of Na0.67Ni0.15Fe0.2Mn0.65O2 (N‐NFM) is prepared through an improved coprecipitation method. Then, the chemical properties of interfaces between the N‐NFM cathode and organic liquid electrolytes based on NaClO4 and NaPF6 are investigated, respectively. Results show that the cathode electrolyte interphase (CEI) film formed in the NaPF6‐based electrolyte is dense and uniform, which inhibits the dissolution of TM ions effectively and provides a low energy barrier for the transport of Na+. Apart from that the CEI film formed in the NaClO4‐based electrolyte contains more organic but less inorganic compounds, resulting in an increase in impedance. In addition, it is believed that the stability of the CEI film is susceptible to the perchlorate with strong oxidizing property. In this role, a small part of the CEI film falls from the cathode surface, accelerating the dissolution of TM ions and leading to the reactivation of electrolyte decomposition.
ObjectiveTo assess the quality of primary healthcare (PHC) for patients with diabetes in China from 2011 to 2015.SettingThis study analysed data on 1006, 1472 and 1771 participants with diabetes who were surveyed in 2011, 2013 and 2015, respectively, in the China Health and Retirement Longitudinal Study, a nationally representative survey conducted in 29 provinces of China.Outcome measuresThe study measured the proportions of patients with diabetes who received diabetes-related health education, examinations and treatments, as well as the hospital admission rate due to diabetes of these patients. Multilevel logistic regression was used to adjust sociodemographic variables.ResultsAccording to the multivariate analysis, the proportion of patients who received diabetes-related health education decreased significantly (OR=0.74, 95% CI 0.61 to 0.90), and the proportion of those receiving examinations and treatments remained unchanged from 2011 to 2015. Diabetes-related hospitalisation increased from 4.01% in 2011 to 6.08% in 2013 (OR=1.47, 95% CI 0.97 to 2.22), and recurrent hospitalisations increased from 18.87% in 2011 to 28.45% in 2015 (OR=1.78, 95% CI 1.44 to 2.20). The proportions of patients with diabetes-related and recurrent hospitalisations in western China were higher than those in the east (OR=1.80, 95% CI 1.13 to 2.87; OR=1.92, 95% CI 1.50 to 2.45).ConclusionsNationally, the analysis of patient-reported process and outcome indicators cannot confirm that the quality of PHC has improved in China during 2011–2015. Regional disparities in primary diabetes care require urgent resource allocation to western China. Establishing a national quality registry for PHC, which transparently reports outcomes by region and social-economic position, is essential for countries sharing the challenge of improving both quality and equity of PHC.
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