The cluster states and Greenberger-Horne-Zeilinger (GHZ) states are two different types of multipartite quantum entangled states. We present the first experimental results generating continuous variable quadripartite cluster and GHZ entangled states of electromagnetic fields. Utilizing two amplitude-quadrature and two phase-quadrature squeezed states of light and linearly optical transformations, the two types of entangled states for amplitude and phase quadratures of light are experimentally produced. The combinations of the measured quadrature variances prove the full inseparability of the generated four subsystems. The presented experimental schemes show that the multipartite entanglement of continuous variables can be deterministically generated with the relatively simple implementation.
Co/Fe Prussian Blue analogues are known to display both thermally and light induced electron transfer attributed to the switching between diamagnetic {Fe(II)LS(μ-CN)Co(III)LS} and paramagnetic {Fe(III)LS(μ-CN)Co(II)HS} pairs (LS = low spin; HS = high spin). In this work, a dinuclear cyanido-bridged Co/Fe complex, the smallest {Fe(μ-CN)Co} moiety at the origin of the remarkable physical properties of these systems, has been designed by a rational building-block approach. Combined structural, spectroscopic, magnetic and photomagnetic studies reveal that a metal-to-metal electron transfer that can be triggered in solid state by light, temperature and solvent contents, is observed for the first time in a dinuclear complex.
An ideal material for C 2 H 6 /C 2 H 4 separation would simultaneously have the highest C 2 H 6 uptake capacity and the highest C 2 H 6 /C 2 H 4 selectivity. But such material is elusive. A benchmark material for ethane-selective C 2 H 6 /C 2 H 4 separation is peroxo-functionalized MOF-74-Fe that exhibits the best known separation performance due to its high C 2 H 6 /C 2 H 4 selectivity (4.4), although its C 2 H 6 uptake capacity is moderate (74.3 cm 3 /g). Here, we report a family of pore-space-partitioned crystalline porous materials (CPMs) with exceptional C 2 H 6 uptake capacity and C 2 H 6 /C 2 H 4 separation potential (i.e., C 2 H 4 recovered from the mixture) despite their moderate C 2 H 6 /C 2 H 4 selectivity (up to 1.75). The ethane uptake capacity as high as 166.8 cm 3 /g at 1 atm and 298 K, more than twice that of peroxo-MOF-74-Fe, has been achieved even though the isosteric heat of adsorption (21.9−30.4 kJ/mol) for these CPMs is as low as about one-third of that for peroxo-MOF-74-Fe (66.8 kJ/mol). While the overall C 2 H 6 /C 2 H 4 separation potentials have not yet surpassed peroxo-MOF-74-Fe, these robust CPMs exhibit outstanding properties including high thermal stability (up to 450 °C) and aqueous stability, low regeneration energy, and a high degree of chemical and geometrical tunability within the same isoreticular framework.
The unconditional entanglement swapping for continuous variables is experimentally demonstrated. Two initial entangled states are produced from two nondegenerate optical parametric amplifiers operating at de-amplification. Through implementing the direct measurement of the Bell-state between two optical beams from each amplifier the remaining two optical beams, which have never directly interacted with each other, are entangled. The quantum correlation degrees of 1.23 and 1.12 dB below the shot noise limit for the amplitude and phase quadratures resulting from the entanglement swapping are measured straightly.
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