Based on a newly developed daily precipitation dataset of 740 stations in China and more robust trend detection techniques, trends in annual and seasonal total precipitation and in extreme daily precipitation, defined as those larger than its 95th percentile for the year, summer, and winter half years, have been assessed for the period 1951–2000. Possible links between changes in total precipitation and frequency of extremes have also been explored. The results indicate that there is little trend in total precipitation for China as a whole, but there are distinctive regional and seasonal patterns of trends. Annual total precipitation has significantly decreased over southern northeast China, north China, and over the Sichuan Basin but significantly increased in western China, the Yangtze River valley, and the southeastern coast. In western China, precipitation increase has been observed for both cold and warm seasons. However, trends differ from one season to another in eastern China. Spring precipitation has increased in southern northeast China and north China but decreased significantly in the midreach of the Yangzte River. The summer precipitation trend is very similar to that of annual totals. Autumn precipitation has generally decreased throughout eastern China. In winter, precipitation has significantly decreased over the northern part of eastern China but increased in the south. The number of rain days has significantly decreased throughout most parts of China with northwest China being an exception. Meanwhile, precipitation intensity has significantly increased. This suggests that the precipitation increase in western China is due to the increase in both precipitation frequency and intensity. In eastern China, the impact of reduced number of rain days seems to be more dominant in the north while the influence of enhanced intensity prevails in the south. Over regions with increasing precipitation trends, there have been much higher than normal frequency of precipitation extreme events. For example, significant increases in extreme precipitation have been found in western China, in the mid–lower reaches of the Yangtze River, and in parts of the southwest and south China coastal area. A significant decrease in extremes is observed in north China and the Sichuan Basin. Trends in the number of extremes and total precipitation from nonextreme events are generally in phase. An exception is southwest China where an increase of extreme events is associated with a decrease in total nonextreme precipitation.

Abstract. Aerosol variations and trends over different land and ocean regions from 1980 to 2009 are analyzed with the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model and observations from multiple satellite sensors and available ground-based networks. Excluding time periods with large volcanic influence, aerosol optical depth (AOD) and surface concentration over polluted land regions generally vary with anthropogenic emissions, but the magnitude of this association can be dampened by the presence of natural aerosols, especially dust. Over the 30-year period in this study, the largest reduction in aerosol levels occurs over Europe, where AOD has decreased by 40–60% on average and surface sulfate concentrations have declined by a factor of up to 3–4. In contrast, East Asia and South Asia show AOD increases, but the relatively high level of dust aerosols in Asia reduces the correlation between AOD and pollutant emission trends. Over major dust source regions, model analysis indicates that the change of dust emissions over the Sahara and Sahel has been predominantly driven by the change of near-surface wind speed, but over Central Asia it has been largely influenced by the change of the surface wetness. The decreasing dust trend in the North African dust outflow region of the tropical North Atlantic and the receptor sites of Barbados and Miami is closely associated with an increase of the sea surface temperature in the North Atlantic. This temperature increase may drive the decrease of the wind velocity over North Africa, which reduces the dust emission, and the increase of precipitation over the tropical North Atlantic, which enhances dust removal during transport. Despite significant trends over some major continental source regions, the model-calculated global annual average AOD shows little change over land and ocean in the past three decades, because opposite trends in different land regions cancel each other out in the global average, and changes over large open oceans are negligible. This highlights the necessity for regional-scale assessment of aerosols and their climate impacts, as global-scale average values can obscure important regional changes.

[1] Based on the daily surface air temperature data from about 200 stations during 1951 -1999 in China, changes in the frequency of some extreme temperature events were studied with a focus on trends. For China as a whole, the number of hot days (Tmax over 35°C) displays a slightly decreasing trend, while the number of frost days (Tmin below 0°C) exhibits a significant decreasing trend. Meanwhile, increasing trends were detected in the frequencies of warm days and warm nights. In addition, decreasing trends was found in the frequencies of cool days and even stronger decreasing trend was found in frequencies of cool nights in China.

Abstract. An assessment of global particulate nitrate and ammonium aerosol based on simulations from nine models participating in the Aerosol Comparisons between Observations and Models (AeroCom) phase III study is presented. A budget analysis was conducted to understand the typical magnitude, distribution, and diversity of the aerosols and their precursors among the models. To gain confidence regarding model performance, the model results were evaluated with various observations globally, including ground station measurements over North America, Europe, and east Asia for tracer concentrations and dry and wet depositions, as well as with aircraft measurements in the Northern Hemisphere mid-to-high latitudes for tracer vertical distributions. Given the unique chemical and physical features of the nitrate occurrence, we further investigated the similarity and differentiation among the models by examining (1) the pH-dependent NH3 wet deposition; (2) the nitrate formation via heterogeneous chemistry on the surface of dust and sea salt particles or thermodynamic equilibrium calculation including dust and sea salt ions; and (3) the nitrate coarse-mode fraction (i.e., coarse/total). It is found that HNO3, which is simulated explicitly based on full O3-HOx-NOx-aerosol chemistry by all models, differs by up to a factor of 9 among the models in its global tropospheric burden. This partially contributes to a large difference in NO3−, whose atmospheric burden differs by up to a factor of 13. The atmospheric burdens of NH3 and NH4+ differ by 17 and 4, respectively. Analyses at the process level show that the large diversity in atmospheric burdens of NO3−, NH3, and NH4+ is also related to deposition processes. Wet deposition seems to be the dominant process in determining the diversity in NH3 and NH4+ lifetimes. It is critical to correctly account for contributions of heterogeneous chemical production of nitrate on dust and sea salt, because this process overwhelmingly controls atmospheric nitrate production (typically > 80 %) and determines the coarse- and fine-mode distribution of nitrate aerosol.