We review the use of hollow-core photonic crystal fibers (PCFs) in the field of ultrafast gas-based nonlinear optics, including recent experiments, numerical modeling, and a discussion of future prospects. Concentrating on broadband guiding kagomé-style hollow-core PCF, we describe its potential for moving conventional nonlinear fiber optics both into extreme regimes-such as few-cycle pulse compression and efficient deep ultraviolet wavelength generation-and into regimes hitherto inaccessible, such as single-mode guidance in a photoionized plasma and high-harmonic generation in fiber.

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Unlike the capillaries conventionally used for gas-based spectral broadening of ultrashort (<100 fs) multi-millijoule pulses, which produce only normal dispersion at usable pressure levels, hollow-core photonic crystal fibres provide pressure-adjustable normal or anomalous dispersion. They also permit low-loss guidance in a hollow channel that is about ten times narrower and has a 100-fold-higher effective nonlinearity than capillary-based systems. This has led to several dramatic results, including soliton compression to few-cycle pulses, widely tunable deep-ultraviolet light sources, novel soliton-plasma interactions and multi-octave Raman frequency combs. A new generation of versatile and efficient gas-based light sources, which are tunable from the vacuum ultraviolet to the near infrared, and of versatile and efficient pulse compression devices is emerging

Although supercontinuum sources are readily available for the visible and near infrared (IR), and recently also for the mid-IR, many areas of biology, chemistry, and physics would benefit greatly from the availability of compact, stable, and spectrally bright deep-ultraviolet and vacuum-ultraviolet (VUV) supercontinuum sources. Such sources have, however, not yet been developed. Here we report the generation of a bright supercontinuum, spanning more than three octaves from 124 nm to beyond 1200 nm, in hydrogen-filled kagome-style hollow-core photonic crystal fiber (kagome-PCF). Few-microjoule, 30 fs pump pulses at wavelength of 805 nm are launched into the fiber, where they undergo self-compression via the Raman-enhanced Kerr effect. Modeling indicates that before reaching a minimum subcycle pulse duration of similar to 1 fs, much less than one period of molecular vibration (8 fs), nonlinear reshaping of the pulse envelope, accentuated by self-steepening and shock formation, creates an ultrashort feature that causes impulsive excitation of long-lived coherent molecular vibrations. These phase modulate a strong VUV dispersive wave (at 182 nm or 6.8 eV) on the trailing edge of the pulse, further broadening the spectrum into the VUV. The results also show for the first time that kagome-PCF guides well in the VUV. (C) 2015 Optical Society of Americ

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