Buoyancy and momentum fluxes are important parameters to determine the plume rise which is related to the ability to dilute air pollutants emitted from combustion stack sources. The change of temperature due to waste heat recovery directly affects these fluxes. This study analyzed buoyancy and momentum fluxes and evaluated the ground level concentration of PM-10 prior and after implementation of waste heat recovery in the area surrounding one of the largest cement production plants in Thailand. The results showed that the ambient temperature was the significant parameter affecting buoyancy and momentum fluxes. The buoyancy flux was found to be the dominant force to the rise of plume for both scenarios. There were no differences in the predicted PM-10 ground level concentrations at receptors around the cement plant for the model simulation under two scenarios. Therefore, it was concluded that decreasing of stack gas exit temperature does not affect the dispersion of air pollutants in the cement industry.
The emission inventory, emission factor, and spatial concentration distribution of volatile organic compounds (VOCs) from a petrochemical industry (aromatics plant) were intensively evaluated in this study to elucidate the potential sources of BTX emission and their contribution to ambient concentrations. Five emission groups were quantified through direct measurement and emission models. These data were then used as input for the AERMOD dispersion model for the source apportionment analysis. The source to ambient contribution analysis revealed that a wastewater treatment facility and organic liquid storage tank were major contributors accounting for about 20.6–88.4% and 10.3–75.4% to BTX environmental concentrations, respectively. The highest annual ambient concentrations of benzene (B), toluene (T), and xylenes (X) were predicted as 9.0, 2.8, and 57.9 µg/m3 at the fence line of the plant boundary, respectively. These findings assist policymakers in prioritizing the appropriate control measures to the right source by considering not just the amount released but also their contribution to ambient concentrations. This study suggested that the wastewater treatment unit should be changed to the closed system which will benefit reduction in its emission (45.05%) as well as effectively minimizing ambient VOC concentration by 49.96% compared to its normal operation.
The purpose of this research was to explicate a human health risk assessment that can be employed with inhalation risk estimates to provide a screening level of risks. Model input parameters provide reasonable values with the site- and compound-specific values relied on by the Human Health Risk Assessment Protocol (HHRAP). This method uses a generic risk assessment, consisting of air dispersion and deposition modeling followed by risk modeling. An intensive evaluation was conducted in the surrounding area of the largest petroleum and petrochemical estate in Thailand, the Maptaphut industrial area, where a large volume of VOCs was emitted, with an increasing negative health impact on the local population. The potential inhalation health risk assessment showed that the lifetime cancer risk in all residential areas is higher than the health benchmarks. The highest cancer risk was 7.82 × 10−2 in children and 3.91 × 10−1 in adults. The inhalation effects are based on the specific emission rates, the united concentrations and deposition fluxes, and the emission phase. The results revealed that four VOCs (benzene, 1,3-butadiene, vinyl chloride, and 1,2-dichloroethane) should be given priority when controlling for sustainable health risk management through the comprehensive analysis of the integrated analysis of air dispersion and health risk mathematical models.
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