Sensor-laden wearable systems that are capable of providing continuous measurement of key physiological parameters coupled with data storage, drug delivery and feedback therapy have attracted huge interest. Here we report a stretchable wireless system for sweat pH monitoring, which is able to withstand up to 53% uniaxial strain and more than 500 cycles to 30% strain. The stretchability of the pH sensor patch is provided by a pair of serpentine-shaped stretchable interconnects. The pH sensing electrode is made of graphite-polyurethane composite, which is suitable for biosensor application. The sensing patch validated through in-depth electrochemical studies, exhibits a pH sensitivity of 11.13 ± 5.8 mV/pH with a maximum response time of 8 s. Interference study of ions and analyte (Na, K and glucose) in test solutions shows negligible influence on the pH sensor performance. The pH data can be wirelessly and continuously transmitted to smartphone through a stretchable radio-frequency-identification antenna, of which the radiating performance is stable under 20% strain, as proved by vector network analyzer measurement. To evaluate the full system, the pH value of a human sweat equivalent solution has been measured and wirelessly transmitted to a custom-developed smart phone App.

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Flexible electronics has huge potential to bring revolution in robotics and prosthetics as well as to bring about the next big evolution in electronics industry. In robotics and related applications, it is expected to revolutionise the way with which machines interact with humans, real-world objects and the environment. For example, the conformable electronic or tactile skin on robot's body, enabled by advances in flexible electronics, will allow safe robotic interaction during physical contact of robot with various objects. Developing a conformable, bendable and stretchable electronic system requires distributing electronics over large non-planar surfaces and movable components. The current research focus in this direction is marked by the use of novel materials or by the smart engineering of the traditional materials to develop new sensors, electronics on substrates that can be wrapped around curved surfaces. Attempts are being made to achieve flexibility/stretchability in e-skin while retaining a reliable operation. This review provides insight into various materials that have been used in the development of flexible electronics primarily for e-skin applications.

This article presents recent progress and a comprehensive overview of stretchable interconnects based on printable nanocomposites. Nanocomposite-based inks for printed stretchable interconnects have been categorized according to dispersed filler materials. They comprise of carbon-based fillers and metal-based fillers. Benefits in terms of excellent electrical performance and elastic properties make nanocomposites the ideal candidates for stretchable interconnect applications. Deeper analysis of nanocomposites-based stretchable interconnects includes the correlation between the size of fillers, percolation ratio, maximum electrical conductivity and mechanical elasticity. The key trends in the field have been highlighted using curve fitting methods on large data collected from the literature. Furthermore, a wide variety of applications for stretchable interconnects are presented.

In this work, we present a potentiometric pH sensor on textile substrate for wearable applications. The sensitive (thick film graphite composite) and reference electrodes (Ag/AgCl) are printed on cellulose-polyester blend cloth. An excellent adhesion between printed electrodes allow the textile-based sensor to be washed with a reliable pH response. The developed textile-based pH sensor works on the basis of electrochemical reaction, as observed through the potentiometric, cyclic voltammetry (100 mV/s) and electrochemical impedance spectroscopic (10 mHz to 1 MHz) analysis. The electrochemical double layer formation and the ionic exchanges of the sensitive electrode-pH solution interaction are observed through the electrochemical impedance spectroscopic analysis. Potentiometric analysis reveals that the fabricated textile-based sensor exhibits a sensitivity (slope factor) of 4 mV/pH with a response time of 5 s in the pH range 6–9. The presented sensor shows stable response with a potential of 47 ± 2 mV for long time (2000 s) even after it was washed in tap water. These results indicate that the sensor can be used for wearable applications.

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Abstract-This work presents a novel stretchable pH sensing patch to detect the pH in body fluid which is one of the most important parameters in human health monitoring. The sensing patch is a hybrid package comprising of polyimide/gold-based stretchable interconnects and graphite composite-based flexible pH sensor. With the integration of stretchable interconnects, the patch is able to withstand external stretching up to 50% longer than its original length. Moreover, the electrical behavior of the patch does not degrade as studied by the real-time resistance investigation. In order to protect the connecting electrodes and wirings from direct contacting with solution under analysis, the sensing patch is encapsulated with elastic polymer with the active sensing area exposed. The fabricated patch reveals a high pH sensitivity of 36.2 µA/pH in the pH range between 5 and 9 which is validated through electrochemical and electroanalytical studies.