To tackle the challenge of the data accuracy issues of low-cost sensors (LCSs), the objective of this work was to obtain robust correction equations to convert LCS signals into data comparable to that of research-grade instruments using side-by-side comparisons. Limited sets of seed LCS devices, after laboratory evaluations, can be installed strategically in areas of interest without official monitoring stations to enable reading adjustments of other uncalibrated LCS devices to enhance the data quality of sensor networks. The robustness of these equations for LCS devices (AS-LUNG with PMS3003 sensor) under a hood and a chamber with two different burnt materials and before and after 1.5 years of field campaigns were evaluated. Correction equations with incense or mosquito coils burning inside a chamber with segmented regressions had a high R2 of 0.999, less than 6.0% variability in the slopes, and a mean RMSE of 1.18 µg/m3 for 0.1–200 µg/m3 of PM2.5, with a slightly higher RMSE for 0.1–400 µg/m3 compared to EDM-180. Similar results were obtained for PM1, with an upper limit of 200 µg/m3. Sensor signals drifted 19–24% after 1.5 years in the field. Practical recommendations are given to obtain equations for Federal-Equivalent-Method-comparable measurements considering variability and cost.
Many low-cost sensors (LCSs) are distributed for air monitoring without any rigorous calibrations. This work applies machine learning with PM2.5 from Taiwan monitoring stations to conduct in-field corrections on a network of 39 PM2.5 LCSs from July 2017 to December 2018. Three candidate models were evaluated: Multiple linear regression (MLR), support vector regression (SVR), and random forest regression (RFR). The model-corrected PM2.5 levels were compared with those of GRIMM-calibrated PM2.5. RFR was superior to MLR and SVR in its correction accuracy and computing efficiency. Compared to SVR, the root mean square errors (RMSEs) of RFR were 35% and 85% lower for the training and validation sets, respectively, and the computational speed was 35 times faster. An RFR with 300 decision trees was chosen as the optimal setting considering both the correction performance and the modeling time. An RFR with a nighttime pattern was established as the optimal correction model, and the RMSEs were 5.9 ± 2.0 μg/m3, reduced from 18.4 ± 6.5 μg/m3 before correction. This is the first work to correct LCSs at locations without monitoring stations, validated using laboratory-calibrated data. Similar models could be established in other countries to greatly enhance the usefulness of their PM2.5 sensor networks.
Household air pollution is one of the leading environmental risk factors for death with particulate matter with an aerodynamic diameter less than or equal to 2.5 μm (PM 2.5 ), a classified human carcinogen, 1 as a major concern. [2][3][4] In particular, Asia accounted for two-thirds of global premature deaths, with 1.64 million in 2017 due to household air pollution, 3,4 while the intensities, frequencies, durations, and contribution of distinct PM 2.5 sources in Asian households have seldom been evaluated. In addition, indoor infiltration of high ambient PM 2.5 levels in Asia 5 affecting Indoor Air Quality (IAQ) exacerbates exposure levels indoors. Characterizing PM 2.5 exposures due to these sources in Asian households is critical for both environmental health research and health advisories to reduce the associated health risks. 6,7 PM 2.5 exposures are usually higher than the ambient levels measured by regulatory monitoring stations. [7][8][9] Distinct sources in Asian households such as cooking and incense burning generate
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