Existing ionic artificial muscles still require a technology breakthrough for much faster response speed, higher bending strain, and longer durability. Here, we report an MXene artificial muscle based on ionically cross-linked Ti3C2Tx with poly(3,4 ethylenedioxythiophene)-poly(styrenesulfonate), showing ultrafast rise time of within 1 s in DC responses, extremely large bending strain up to 1.37% in very low input voltage regime (0.1 to 1 V), long-term cyclic stability of 97% up to 18,000 cycles, markedly reduced phase delay, and very broad frequency bandwidth up to 20 Hz with good structural reliability without delamination under continuous electrical stimuli. These artificial muscles were successfully applied to make an origami-inspired narcissus flower robot as a wearable brooch and dancing butterflies and leaves on a tree as a kinetic art piece. These successful demonstrations elucidate the wide potential of MXene-based soft actuators for the next-generation soft robotic devices including wearable electronics and kinetic art pieces.

MXenes, a member of 2D inorganic compounds that contain few-atom-thick layers of transition metal carbides, nitrides, and polar surface functional groups, are extraordinary materials for many applications including stimuliresponsive actuators. Here, an extensive review on MXene-based actuators in comparison with other 2D materials-based actuators is reported, highlighting the main differences in view of chemical structure, mechanical properties, and electrical functionalities. First, since MXenes are newcomers in the field of actuators, their properties are explained including cation and ionic liquid intercalation, high capacitance, good electrical and thermal conductivity, excellent electromagnetic wave absorption, hydrophilicity, and outstanding dispersion in many polar solvents. Second, electro-ionic, electrochemical, electrothermal, photothermal, and humidity-responsive MXene-based actuators are comprehensively addressed with detailed actuation mechanisms, focusing on electro-ionic soft actuators. Third, several applications of those actuators are summarized with an emphasis on soft robotics and future directions of MXene-based actuators are suggested.

Future smart mobile electronics and wearable robotics that can perform delicate activities controlled by artificial intelligence can require rapid motion actuators working at low voltages with acceptable safety and improved energy efficiency. Accordingly, ionic soft actuators can have great potential over other counterparts because they exhibit gentle movements at low voltages, less than 2 V. However, these actuators currently show deficient performances at sub‐1 V voltages in the high‐frequency range because of the lack of electrode materials with the vital antagonistic properties of high capacitance and good conductivity. Herein, a mutually exclusive nanohybrid electrode (pMoS2‐nSNrGO) is reported consisting of oxide‐doped p‐type molybdenum‐disulfide and sulfur‐nitrogen‐codoped n‐type reduced‐graphene‐oxide. The pMoS2‐nSNrGO electrode derives high capacitance from MoS2 and good charge transfer between the two components from p‐n nano‐junctions, resulting in excellent actuation performances (670% improvement compared with rGO electrode at 0.5 V and 1 Hz, together with fast responses up to 15 Hz). With such excellent performances, these actuators can be successfully applied to realize an artificial soft robotic finger system for delicately touching the fragile surfaces of smartphones and tablets. The mutually exclusive pMoS2‐nSNrGO electrode can open a new way to develop high‐performance soft actuators for soft robotic applications in the future.

Ionic soft actuators, which exhibit large mechanical deformations under low electrical stimuli, are attracting attention in recent years with the advent of soft and wearable electronics. However, a key challenge for making highperformance ionic soft actuators with large bending deformation and fast actuation speed is to develop a stretchable and flexible electrode having high electrical conductivity and electrochemical capacitance. Here, a functionally antagonistic hybrid electrode with hollow tubular graphene meshes and nitrogen-doped crumpled graphene is newly reported for superior ionic soft actuators. Three-dimensional network of hollow tubular graphene mesh provides high electrical conductivity and mechanically resilient functionality on whole electrode domain. On the contrary, nitrogen-doped wrinkled graphene supplies ultrahigh capacitance and stretchability, which are indispensably required for improving electrochemical activity in ionic soft actuators. Present results show that the functionally antagonistic hybrid electrode greatly enhances the actuation performances of ionic soft actuators, resulting in much larger bending deformation up to 620%, ten times faster rise time and much lower phase delay in a broad range of input frequencies. This outstanding enhancement mostly attributes to exceptional properties and synergistic effects between hollow tubular graphene mesh and nitrogen-doped crumpled graphene, which have functionally antagonistic roles in charge transfer and charge injection, respectively.

Treebank is an important resource for both research and application of natural language processing. For Vietnamese, we still lack such kind of corpora. This paper presents up-to-date results of a project for Vietnamese treebank construction. Since Vietnamese is an isolating language and has no word delimiter, there are many ambiguities in sentence analysis. We systematically applied a lot of linguistic techniques to handle such ambiguities. Annotators are supported by automaticlabeling tools and a tree-editor tool. Raw texts are extracted from Tuoi Tre (Youth), an online Vietnamese daily newspaper. The current annotation agreement is around 90 percent.